留言板

尊敬的读者、作者、审稿人, 关于本刊的投稿、审稿、编辑和出版的任何问题, 您可以本页添加留言。我们将尽快给您答复。谢谢您的支持!

姓名
邮箱
手机号码
标题
留言内容
验证码

东海和黄海冬季海水中二甲亚砜的分布及影响因素

王 鑫 张洪海 杨桂朋

王 鑫, 张洪海, 杨桂朋. 东海和黄海冬季海水中二甲亚砜的分布及影响因素[J]. 环境科学研究, 2014, 27(10): 1119-1125.
引用本文: 王 鑫, 张洪海, 杨桂朋. 东海和黄海冬季海水中二甲亚砜的分布及影响因素[J]. 环境科学研究, 2014, 27(10): 1119-1125.
WANG Xin, ZHANG Hong-hai, YANG Gui-peng. Distribution of Dimethylsulfoxide and Its Influencing Factors in the East China Sea and the Yellow Sea in Winter[J]. Research of Environmental Sciences, 2014, 27(10): 1119-1125.
Citation: WANG Xin, ZHANG Hong-hai, YANG Gui-peng. Distribution of Dimethylsulfoxide and Its Influencing Factors in the East China Sea and the Yellow Sea in Winter[J]. Research of Environmental Sciences, 2014, 27(10): 1119-1125.

东海和黄海冬季海水中二甲亚砜的分布及影响因素

基金项目: 国家自然科学基金项目(41030858,41320104008,41306069)

Distribution of Dimethylsulfoxide and Its Influencing Factors in the East China Sea and the Yellow Sea in Winter

  • 摘要: 于2011年12月—2012年1月对我国东海、黄海表层及不同深度海水中c(DMSOd)(DMSOd为溶解态二甲亚砜)和c(DMSOp)(DMSOp为颗粒态二甲亚砜)的分布进行了研究,并探讨了其来源及影响因素. 结果表明:表层海水中c(DMSOd)和c(DMSOp)分别为(10.10±7.54)和(8.72±7.80) nmol/L,其水平分布明显受调查海域中浮游植物组成和丰度的影响;垂直分布上,c(DMSOd)和c(DMSOp)的最大值均出现在浅水层(3~20 m). 相关分析表明,c(DMSOd)与c(DMS)(DMS为二甲基硫)之间没有相关性,但与c(DMSOp)显著相关(R=0.442, n=41, P<0.006),说明冬季表层海水中DMSOd主要来源于浮游植物细胞内DMSO的释放,而不是DMS的氧化(光化学氧化和微生物氧化). 另外,c(DMSOp)/ρ(Chla)与盐度呈正相关(R=0.532, n=46, P<0.004),说明盐度的改变会影响浮游植物组成的变化,进而影响c(DMSOp).

     

  • [1] DEL VALLE D A,KIEBER D J,TOOLE D A,et al.Dissolved DMSO production via biological and photochemical oxidation of dissolved DMS in the Ross Sea,Antarctica.Deep-Sea Research Ⅰ,2009,6:166-177.
    [2] HATTON A D,TURNER S M,MALIN G,et al.Dimethylsulphoxide and other biogenic sulphur compounds in the Galapagos Plume.Deep-Sea Research Ⅱ,1998,5:1043-1053.
    [3] YANG G P,WANG X,ZHANG H H,et al.Temporal and spatial variations of dimethylsulfoxide in the Bohai Sea and the Yellow Sea.Journal of Sea Research,2014,0:33-43.
    [4] RIDGEWAY R G,THORNTON D C,BANDY A R.Determination of trace aqueous dimethylsulfoxide concentrations by isotope dilution gas chromatography/mass spectrometry:application to rain and sea water.Journal of Atmospheric Chemistry,1992,4:53-60.
    [5] ANDREAE M O.Dimethylsulfoxide in marine and freshwaters.Limnology and Oceanography,1980,5(6):1054-1063.
    [6] BERRESHEIM H,EISELE F L,TANNER D J,et al.Atmospheric sulfur chemistry and CCN concentrations over the Northeastern Pacific coast.Journal of Geophysical Research,1993,8(D7):12701-12711.
    [7] CHARLSON R J,LOVELOCKL J E,ANDREAE M O,et al.Oceanic phytoplankton,atmospheric sulphur,cloud albedo and climate.Nature,1987,6:655-661.
    [8] 杜晓明,刘厚田,柳若安,等.厦门近海海域海水二甲基硫排放通量的研究.环境科学研究,1998,1(2):34-36.DU Xiaoming,LIU Houtian,LIU Ruoan,et al.The flux of oceanic dimethyl sulfide from coastal area in Xiamen to the atmosphere.Research o f Environmental Sciences,1998,1(2):34-36.
    [9] BRIMBLECOMBE P,SHOOTER D.Photo-oxidation of dimethylsulphide in aqueous solution.Marine Chemistry,1986,9(4):343-353.
    [10] ZHANG L,KUNIYOSHI I,HIRAI M,et al.Oxidation of dimethyl sulfide by Pseudomonas acidovorans DMR-11 isolated from peat biofilter.Biotechnology Letters,1991,3(3):223-228.
    [11] SIM R,HATTON A D,MALIN G,et al.Particulate dimethyl sulphoxide in sea water:production by microplankton.Marine Ecology Progress Series,1998,7:291-296.
    [12] SPIESE C E,KIEBER D J,NOMURA C T,et al.Reduction of dimethylsulfoxide to dimethylsulfide by marine phytoplankton.Limnology and Oceanography,2009,4(2):560-570.
    [13] DE MORA S J,LEE P A,GROUT A,et al.Aspects of the biogeochemistry of sulfur in glacial melt water ponds on the McMurdo Ice Shelf,Antarctica.Antarctic Science,1996,8(1):15-22.
    [14] BODEN R,MURRELL J C,SCHAFER H.Dimethylsulfide is an energy source for the heterotrophic marine bacterium Sagittula stellata.FEMS Microbiology Letters,2011,2(2):188-193.
    [15] HATTON A D,SHENOY D M,HART M C,et al.Metabolism of DMSP,DMS and DMSO by thecultivable bacterial community associated with the DMSP-producing dinoflagellate Scrippsiella trochoidea.Biogeochemistry,2012,0:131-146.
    [16] 李猛,袁东星,汤坤贤.围隔藻类水华演替过程中二甲基硫化物的含量动态.生态学报,2007,7 (12):5308-5317.LI Meng,YUAN Dongxing,TANG Kunxian.Variations of the concentration of dimethyl sulfur compounds during three algal blooms in a mesocosm experiment.Acta Ecologica Sinica,2007,7(12):5308-5317.
    [17] 孙倩,金晓英,李猛,等.厦门西海域典型站位二甲基硫化物周日变化初探.环境化学,2006,5 (3):351-355.SUN Qian,JIN Xiaoying,LI Meng,et al.Diel variations of dimethyl sulfur compounds in the surfacewater of Xiamen western sea area.Environmental Chemistry,2006,5(3):351-355.
    [18] 王敏,张洪海,杨桂朋.夏季黄渤海表层海水中二甲亚砜(DMSO)的浓度分布.环境科学,2013,4(1):45-50.WANG Min,ZHANG Honghai,YANG Guipeng.Distribution of dimethylsulfoxide (DMSO) in the surface water of the Yellow Sea and the Bohai Sea.Environmenta Science,2013,4(1):45-50.
    [19] YANG J,YANG G P,YANG J.Study on the analysis and distribution of dimethylsulfoxide in the Jiaozhou Bay.Acta Oceanologica Sinica,2011,0(6):36-45.
    [20] DACEY J W H,BLOUGH N V.Hydroxide decomposition of dimethylsulfoniopropionate to form dimethylsulfide.Geophysical Research Letters,1987,4:1246-1249.
    [21] ZHANG H H,YANG G P,ZHU T.Distribution and cycling of dimethylsulfide (DMS) and dimethylsulfoniopropionate (DMSP) in the sea-surface microlayer of the Yellow Sea,China,in spring.Continental Shelf Research,2008,8(12):2417-2427.
    [22] 张洪海,杨桂朋.胶州湾及青岛近海微表层与次表层中二甲基硫(DMS)与二甲巯基丙酸(DMSP)的浓度分布.海洋与湖沼,2010,1(5):683-691.ZHANG Honghai,YANG Guipeng.Distribution of dimethylsulfide (DMS) and dimethylsulphoniopropionate (DMSP) in the microlayer and subsurface water in Jiaozhou Bay and Qingdao coastal water.Oceanologia et Limnologia Sinica,2010,1(5):683-691.
    [23] YANG G P,LEVASSEUR M,MICHAUD S,et al.Distribution of dimethylsulfide and dimethylsulfoniopropionate and its relation with phytoneuston in the surface microlayer of the western North Atlantic during summer.Biogeochemistry,2009,4(3):243-254.
    [24] SIM R.Trace chromatographic analysis of dimethyl sulfoxide and related methylated sulfur compounds in natural waters.Journal of Chromatography A,1998,7(2):151-164.
    [25] DEL VALLE D A,KIEBER D J,KIENE R P.Depth-dependent fate of biologically-consumed dimethylsulfide in the Sargasso Sea.Marine Chemistry,2007,3:197-208.
    [26] DEL VALLE D A,KIEBER D J,BISGROVE J,et al.Light-stimulated production of dissolved DMSO by a particle-associated process in the Ross Sea,Antarctica.Limnology and Oceanography,2007,2(6):2456-2466.
    [27] HATTON A D.DMSP removal and DMSO production in sedimenting particulate matter in the northern North Sea.Deep-Sea Research Part Ⅱ,2002,9:3053-3065.
    [28] BOUILLON R C,LEE P A,DE MORA S J,et al.Vernal distribution of dimethylsulphide,dimethylsolphoniopropionate,and dimethylsulpoxide in the North Water in 1998.Deep-Sea Research Ⅱ,2002,9:5171-5189.
    [29] SIM R,VILA-COSTA M.Ubiquity of algal dimethylsulfoxide in the surface ocean:geographic and temporal distribution patterns.Marine Chemistry,2006,0:136-146.
    [30] HATTON A D,WILAON S T.Particulate dimethylsulphoxide and dimethylsulphoniopropionate in phytoplankton cultures and Scottish coastal waters.Aquatic Sciences-Research Across Boundaries,2007,9:330-340.
    [31] TOOLE D A,KIEBER D J,KIENE R P,et al.Photolysis and the dimethyl sulfide (DMS) summer paradox in the Sargasso Sea.Limnology Oceanography,2003,8(3):1088-1100.
    [32] HATTON A D.Influence of photochemistry on the cycling of dimethylsulphide in the northern North Sea.Deep-Sea Research Ⅱ,2002,9(15):3039-3052.
    [33] TOOLE D A,KIEBER D J,KIENE R P,et al.High dimethylsulfide photolysis rates in nitrate-rich Antarctic waters.Geophysical Research Letters,2004,doi: 10.1029/2004GL019863.
    [34] BOUILLON R C,MILLER W L.Determination of apparent quantum yield spectra of DMS photo-degradation in an in situ iron-induced north east Pacific Ocean bloom.Geophysical Research Letters,2004,doi: 10.1029/2004GL019536.
  • 加载中
计量
  • 文章访问数:  2102
  • HTML全文浏览量:  24
  • PDF下载量:  134
  • 被引次数: 0
出版历程
  • 收稿日期:  2013-11-15
  • 修回日期:  2014-03-24
  • 刊出日期:  2014-10-25

目录

    /

    返回文章
    返回