【PM2.5与臭氧协同控制专题】编者按:当前,PM2.5和臭氧已经成为影响我国环境空气质量的主要污染物. 2021年3月,第十三届全国人民代表大会第四次会议批准了《中华人民共和国国民经济和社会发展第十四个五年规划和2035年远景目标纲要》,该纲要明确提出要加强城市大气质量达标管理,推进PM2.5和臭氧协同控制,地级及以上城市PM2.5浓度下降10%,有效遏制臭氧浓度增长趋势,基本消除重污染天气. 2021年11月,中共中央、国务院印发《关于深入打好污染防治攻坚战的意见》,明确要求到2025年,臭氧浓度增长趋势得到有效遏制,实现PM2.5和臭氧协同控制. PM2.5和臭氧的协同控制,成为我国“十四五”及更长时期大气污染防治的一项重要任务. 近期,各有关方面围绕PM2.5与臭氧协同控制开展了大量工作,并取得了一定的成果. 有鉴于此,本刊特开设“PM2.5与臭氧协同控制”专栏,经严格的同行评议后,共刊发11篇文章,内容涵盖PM2.5与臭氧的污染特征、相互关系、成因分析、防控理论等方面,以期能引起学界的进一步思考与探讨.
Preliminary Research on Theoretical Framework of Cooperative Control of Air Pollution in China
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摘要: 我国大气污染防治工作在“十三五”期间取得了可喜成绩,PM2.5浓度及重污染天数大幅降低,与此同时,我国城市地区臭氧(O3)污染问题凸显,说明我国大气污染格局发生了深刻变化. 当前,PM2.5与O3成为影响我国城市和区域空气质量的主要因子,二者的协同控制是我国持续改善空气质量的焦点,也成为我国“十四五”期间大气污染防治工作的重点. 本文通过对国内外PM2.5和O3协同控制进展的梳理,总结我国大气复合污染协同治理的现状与挑战,从协同防控目标、核心协同任务、重点支撑保障等角度提出大气复合污染协同治理的理论框架,并对我国PM2.5与O3协同控制工作提出以下几点建议:①坚持科学精准治气;②坚持综合系统治气;③坚持严格依法治气;④坚持多维协同治气.Abstract: During the ‘13th Five-Year Plan’ period, China has made promising achievements in air pollution prevention and control. The concentration of PM2.5 and the number of heavily pollution days have decreased significantly. At the same time, O3 pollution in urban areas has become a prominent problem, indicating that China's air pollution has undergone profound changes. In recent years, PM2.5 and O3 have gradually become the main factors that affect the continuous improvement of air quality in urban and regional areas in China. The so-called complex air pollution of PM2.5 and O3 will be the focused issue of air pollution prevention and control strategy in China and the synergistic control of multiple air pollutants will become the major task during the ‘14th Five-Year Plan’ period. Through combing the progress of synergistic control of the pollutants of PM2.5 and O3 in China and abroad, this paper summarizes the current situation and challenges of the synergistic control of PM2.5 and O3 pollution all over China. We propose a preliminary theoretical framework for collaborative control of air pollution, which includes the objectives of collaborative prevention and control, major tasks and key supporting conditions. In conclusion, we put forward some relevant suggestions for the collaborative control of PM2.5 and O3 pollution: (1) Insist on scientific and precise strategy of air quality. (2) Insist on comprehensive and systematic strategy of air quality. (3) Insist on strict strategy of air quality according to the law. (4) Insist on multi-dimensional coordinated strategy.
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Key words:
- PM2.5 /
- ozone (O3) /
- compound air pollution /
- synergistic control /
- theoretical system
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[1] 生态环境部.中国空气质量改善报告(2013—2018年)[R].北京:生态环境部,2019:1-5. [2] WANG P F,GUO H,HU J L,et al.Responses of PM2.5 and O3 concentrations to changes of meteorology and emissions in China[J].Science of the Total Environment,2019,662:297-306. doi: 10.1016/j.scitotenv.2019.01.227 [3] LI K,JACOB D J,LIAO H,et al.Anthropogenic drivers of 2013-2017 trends in summer surface ozone in China[J].Proceedings of the National Academy of Sciences of the United States of America,2019,116(2):422-427. doi: 10.1073/pnas.1812168116 [4] LYU X P,WANG N,GUO H,et al.Causes of a continuous summertime O3 pollution event in Jinan,a central city in the North China Plain[J].Atmospheric Chemistry and Physics,2019,19(5):3025-3042. doi: 10.5194/acp-19-3025-2019 [5] QU Y W,WANG T J,CAI Y F,et al.Influence of atmospheric particulate matter on ozone in Nanjing,China:observational study and mechanistic analysis[J].Advances in Atmospheric Sciences,2018,35(11):1381-1395. doi: 10.1007/s00376-018-8027-4 [6] TAN Z F,LU K D,JIANG M Q,et al.Exploring ozone pollution in Chengdu,southwestern China:a case study from radical chemistry to O3-VOC-NOx sensitivity[J].Science of the Total Environment,2018,636:775-786. doi: 10.1016/j.scitotenv.2018.04.286 [7] Nature Geoscience.Cleaner air for China[J].Nature Geoscience,2019,12(7):497. doi: 10.1038/s41561-019-0406-7 [8] 秦思达,王帆,王堃,等.基于WRF-CMAQ模型的辽宁中部城市群PM2.5化学组分特征[J].环境科学研究,2021,34(6):1277-1286.QIN S D,WANG F,WANG K,et al.Numerical simulation study on chemical composition of PM2.5 in urban agglomeration of central Liaoning Province according to WRF-CMAQ model[J].Research of Environmental Sciences,2021,34(6):1277-1286. [9] HU J L,WU L,ZHENG B,et al.Source contributions and regional transport of primary particulate matter in China[J].Environmental Pollution,2015,207:31-42. doi: 10.1016/j.envpol.2015.08.037 [10] 李红,彭良,毕方,等.我国PM2.5与臭氧污染协同控制策略研究[J].环境科学研究,2019,32(10):1763-1778.LI H,PENG L,BI F,et al.Strategy of coordinated control of PM2.5 and ozone in China[J].Research of Environmental Sciences,2019,32(10):1763-1778. [11] 邵平,辛金元,安俊琳,等.长三角工业区夏季近地层臭氧和颗粒物污染相互关系研究[J].大气科学,2017,41(3):618-628.SHAO P,XIN J Y,AN J L,et al.An analysis on the relationship between ground-level ozone and particulate matter in an industrial area in the Yangtze River Delta during summer time[J].Chinese Journal of Atmospheric Sciences,2017,41(3):618-628. [12] XING J,WANG J D,MATHUR R,et al.Impacts of aerosol direct effects on tropospheric ozone through changes in atmospheric dynamics and photolysis rates[J].Atmospheric Chemistry and Physics,2017,17(16):9869-9883. doi: 10.5194/acp-17-9869-2017 [13] XU J,ZHANG Y H,ZHENG S Q,et al.Aerosol effects on ozone concentrations in Beijing:a model sensitivity study[J].Journal of Environmental Sciences,2012,24(4):645-656. doi: 10.1016/S1001-0742(11)60811-5 [14] 苏维瀚,沈济,张秋彭,等.天津地区大气污染状况和气溶胶硫酸盐的研究[J].环境科学学报,1982,2(4):329-341.SU W H,SHEN J,ZHANG Q P,et al.A study of air pollution and aerosol sulfate in the region of Tianjin[J].Acta Scientiae Circumstantiae,1982,2(4):329-341. [15] SAATHOFF H,NAUMANN K H,MÖHLER O,et al.Temperature dependence of yields of secondary organic aerosols from the ozonolysis of α-pinene and limonene[J].Atmospheric Chemistry and Physics,2009,9(5):1551-1577. doi: 10.5194/acp-9-1551-2009 [16] LI J,WANG Z,WANG X,et al.Impacts of aerosols on summertime tropospheric photolysis frequencies and photochemistry over central eastern China[J].Atmospheric Environment,2011,45(10):1817-1829. doi: 10.1016/j.atmosenv.2011.01.016 [17] 张明棣,云龙,李成柳,等.基于观测模型量化VOCs对深圳市城区臭氧生成的影响[J].环境科学研究,2021,34(11):2599-2608.ZHANG M D,YUN L,LI C L,et al.Quantifying impacts of VOCs on ozone formation in urban area of Shenzhen based on observation-based model[J].Research of Environmental Sciences,2021,34(11):2599-2608. [18] LOU S J,LIAO H,ZHU B.Impacts of aerosols on surface-layer ozone concentrations in China through heterogeneous reactions and changes in photolysis rates[J].Atmospheric Environment,2014,85:123-138. doi: 10.1016/j.atmosenv.2013.12.004 [19] 刘艳菊,杨峥,刘庆阳,等.北京4个功能区春冬季大气重污染期间PM10和PM2.5化学污染特征及影响因素分析[J].环境工程技术学报,2021,11(4):631-646. doi: 10.12153/j.issn.1674-991X.20200214LIU Y J,YANG Z,LIU Q Y,et al.Chemical pollution characteristics of PM10 and PM2.5 during heavy air pollution in spring and winter in four functional areas of Beijing and their associated influencing factors[J].Journal of Environmental Engineering Technology,2021,11(4):631-646. doi: 10.12153/j.issn.1674-991X.20200214 [20] FUZZI S,BALTENSPERGER U,CARSLAW K,et al.Particulate matter,air quality and climate:lessons learned and future needs[J].Atmospheric Chemistry and Physics,2015,15(14):8217-8299. doi: 10.5194/acp-15-8217-2015 [21] LEE A K Y.Haze formation in China:importance of secondary aerosol[J].Journal of Environmental Sciences (China),2015,33:261-262. doi: 10.1016/j.jes.2015.06.002 [22] 唐孝炎,张远航,邵敏.大气环境化学[M].2版.北京:高等教育出版社,2006:101-121. [23] Clean Air Asia.Breakthroughs China's path to clean air 2013-2017[R].Beijing:Clean Air Asia,2018. [24] 柴发合.中国未来三年大气污染治理形势预判与对策分析[J].中国环境监察,2019(1):29-31. [25] 张远航,王金南.发达国家有哪些大气治理经验值得我们借鉴[N/OL].北京:中国环境报,(2017-03-03)[2021-09-13].https://www.cenews.com.cn/news/201703/t20170303_823825.html. [26] 薛志钢,郝吉明,陈复,等.国外大气污染控制经验[J].重庆环境科学,2003(11):159-161. [27] 柴发合,王晓,罗宏,等.美国与欧盟关于PM2.5和臭氧的监管政策述评[J].环境工程技术学报,2013,3(1):46-52. doi: 10.3969/j.issn.1674-991X.2013.01.009CHAI F H,WANG X,LUO H,et al.Review of supervision policies of USA and european union on PM2.5 and O3[J].Journal of Environmental Engineering Technology,2013,3(1):46-52. doi: 10.3969/j.issn.1674-991X.2013.01.009 [28] 杜譞,李宏涛.欧美经验对我国“十三五”大气污染防治战略的启示[J].中国环境管理,2016,8(5):57-62.DU X,LI H T.European and American experiences and its implications on air pollution control strategy in China during the ‘13th Five-Year Period’[J].Chinese Journal of Environmental Management,2016,8(5):57-62. [29] Department for Environment,Food & Rural Affairs.The air quality strategy for England,Scotland,Wales and Northern Ireland (Volume 1)[R].England:Department for Environment,Food & Rural Affairs,2007. [30] CHEN D,LI Q B,STUTZ J,et al.WRF-Chem simulation of NOx and O3 in the L.A.basin during CalNex-2010[J].Atmospheric Environment,2013,81:421-432. doi: 10.1016/j.atmosenv.2013.08.064 [31] 李红,鲍捷萌,毕方,等.PM2.5与臭氧污染协同控制:挑战与应对[J].世界环境,2020(5):24-29.LI H,BAO J M,BI F,et al.Synergistic control of PM2.5 and ozone pollution:challenges and responses[J].World Environment,2020(5):24-29. [32] CHENG Y F,ZHENG G J,WEI C,et al.Reactive nitrogen chemistry in aerosol water as a source of sulfate during haze events in China[J].Science Advances,2016,2(12):e1601530. doi: 10.1126/sciadv.1601530 [33] 柴发合.我国大气污染治理历程回顾与展望[J].环境与可持续发展,2020,45(3):5-15.CHAI F H.Review and prospect on the atmospheric pollution control in China[J].Environment and Sustainable Development,2020,45(3):5-15. -