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2015—2020年山西省空气质量时空变化特征及其驱动因素分析

何向阳 张凤英 何立环 马广文 林兰钰 方德昆

何向阳, 张凤英, 何立环, 马广文, 林兰钰, 方德昆. 2015—2020年山西省空气质量时空变化特征及其驱动因素分析[J]. 环境科学研究, 2023, 36(10): 1870-1881. doi: 10.13198/j.issn.1001-6929.2023.08.03
引用本文: 何向阳, 张凤英, 何立环, 马广文, 林兰钰, 方德昆. 2015—2020年山西省空气质量时空变化特征及其驱动因素分析[J]. 环境科学研究, 2023, 36(10): 1870-1881. doi: 10.13198/j.issn.1001-6929.2023.08.03
HE Xiangyang, ZHANG Fengying, HE Lihuan, MA Guangwen, LIN Lanyu, FANG Dekun. Spatiotemporal Variation Characteristics and Driving Factors of Air Quality in Shanxi Province from 2015 to 2020[J]. Research of Environmental Sciences, 2023, 36(10): 1870-1881. doi: 10.13198/j.issn.1001-6929.2023.08.03
Citation: HE Xiangyang, ZHANG Fengying, HE Lihuan, MA Guangwen, LIN Lanyu, FANG Dekun. Spatiotemporal Variation Characteristics and Driving Factors of Air Quality in Shanxi Province from 2015 to 2020[J]. Research of Environmental Sciences, 2023, 36(10): 1870-1881. doi: 10.13198/j.issn.1001-6929.2023.08.03

2015—2020年山西省空气质量时空变化特征及其驱动因素分析

doi: 10.13198/j.issn.1001-6929.2023.08.03
基金项目: 国家重点研发计划项目(No.2022YFC3702604)
详细信息
    作者简介:

    何向阳(1998-),男,山西临汾人,hexyes@outlook.com

    通讯作者:

    方德昆(1990-),男,北京人,工程师,硕士,主要从事生态环境综合分析研究,fangdk@cnemc.cn

  • 中图分类号: X823

Spatiotemporal Variation Characteristics and Driving Factors of Air Quality in Shanxi Province from 2015 to 2020

Funds: National Key Research and Development Program of China (No.2022YFC3702604)
  • 摘要: 山西省是近年来我国空气质量较差的地区之一,本文基于山西省11个地级市2015—2020年空气质量监测结果、气象数据以及2020年的社会经济数据,综合地理加权回归(GWR)模型、多尺度地理加权回归(MGWR)模型以及小波分析等方法开展该地区空气质量时空变化和驱动因素研究. 结果表明:①近年来,山西省SO2、CO和PM2.5浓度均呈明显下降趋势,但NO2和O3污染加重导致山西省空气污染防治形势严峻. ②冬季山西省空气质量空间差异性明显,11个城市中大同市的空气质量最好,临汾市空气质量最差. ③山西省不同社会经济因子与空气污染物相关关系的空间异质性不同,人均GDP和城市绿化覆盖率对SO2浓度影响的空间异质性较高,人均GDP和人口密度对NO2浓度影响的空间异质性较高. ④临汾市、大同市气象因子与PM2.5浓度的相关性一致,两市平均气温与O3浓度均呈显著正相关,风速、降水量和平均相对湿度与O3浓度相关性均较弱,且在两市中存在明显差异. ⑤小波分析结果表明,临汾市、大同市PM2.5浓度与风速在短周期中多呈负相关关系,长周期中PM2.5浓度变化滞后于风速;O3浓度与风速在不同短周期中的相关性不同,长周期中风速变化滞后于O3浓度变化. 研究显示,山西省空气质量持续改善,不同经济因素和气象因素对空气质量时空特征的影响存在明显差异.

     

  • 图  1  山西省海拔及空气质量监测点位

    Figure  1.  Air quality monitoring points and altitude in Shanxi Province

    图  2  2015—2020年山西省六项污染物浓度逐日变化情况

    Figure  2.  Daily concentration of six pollutants in Shanxi Province from 2015 to 2020

    图  3  山西省六项污染物浓度逐年变化特征以及2020年与2015年污染物年均浓度差值

    Figure  3.  Annual characteristics of six pollutant and the difference in annual average concentration difference in Shanxi Province between 2020 and 2015

    图  4  2015—2020年山西省11个地级市的AQI值逐日变化特征

    Figure  4.  Daily characteristics of AQI values in 11 cities of Shanxi Province from 2015 to 2020

    图  5  2015—2020年山西省11个地级市空气质量等级分布情况

    Figure  5.  Air quality grade distribution of 11 cities in Shanxi Province from 2015 to 2020

    图  6  MGWR模型回归系数分布

    Figure  6.  Distribution of MGWR regression coefficient

    图  7  临汾市和大同市PM2.5浓度、O3浓度、风速的小波图

    注:黑实线包围的黄色部分表示相关性通过95%显著检验,阴影部分受到边界效应影响,其功率谱不予考虑[33]. 下同.

    Figure  7.  Wavelet diagram of PM2.5 concentration, O3 concentration and wind speed in Linfen City and Datong City

    图  8  临汾市和大同市PM2.5浓度、O3浓度与风速的交叉小波图、小波相干图

    注:箭头方向朝左表示二者反相位变化,为负相关性,反之亦然.

    Figure  8.  Cross wavelet and wavelet coherence diagram of PM2.5 concentration, O3 concentration and wind speed in Linfen City and Datong City

    表  1  OLS和GWR模型分析结果

    Table  1.   Analysis results of OLS and GWR models

    因变量自变量OLS模型GWR模型
    回归系数PVIF值回归系数最小值回归系数中值回归系数最大值
    SO2浓度 人口密度 −1.289*** 0.005 2.867 −1.312 −1.279 −1.260
    城镇化率 1.370*** 0.002 2.443 1.351 1.354 1.377
    人均GDP −0.046 0.808 1.852 −0.062 −0.037 −0.027
    工业用电量 −0.095 0.584 1.261 −0.106 −0.092 −0.083
    城市绿化覆盖率 0.301 0.111 1.480 0.290 0.297 0.308
    AICc1) 11.699 33.681
    R2 0.895 0.906
    调整R2 0.790 0.741
    F-statistic2) 8.505** 0.017 4
    带宽 17
    NO2浓度 人口密度 0.336 0.427 2.867 0.299 0.343 0.379
    城镇化率 0.203 0.570 2.443 0.183 0.206 0.225
    人均GDP 0.298 0.304 1.852 0.265 0.282 0.319
    工业用电量 −0.151 0.545 1.261 −0.151 −0.145 −0.137
    城市绿化覆盖率 −0.526* 0.065 1.480 −0.525 −0.520 −0.512
    AICc1) 19.717 41.626
    R2 0.759 0.785
    调整R2 0.518 0.411
    F-statistic2) 3.146 0.117
    带宽 17
    注:1)AICc值是衡量模型优良度的一种标准,值越小,模型拟合优度越高. 2) F -statistic用于检验模型是否具有显著性. ***、**、*分别表示在1%、5%、10%水平上的显著性. 下同.
    下载: 导出CSV

    表  2  MGWR模型分析结果

    Table  2.   Analysis results of MGWR model

    因变量自变量MGWR
    回归系数
    最小值
    回归系数
    中值
    回归系数
    最大值
    带宽
    SO2浓度 人口密度 −1.318 −1.314 −1.313 10
    城镇化率 1.314 1.320 1.340 10
    人均GDP −0.072 0.024 0.110 7
    工业用电量 −0.116 −0.103 −0.096 10
    城市绿化覆盖率 0.256 0.302 0.337 8
    AICc 47.603
    R2 0.934
    调整R2 0.766
    NO2浓度 人口密度 0.420 0.463 0.477 9
    城镇化率 0.132 0.158 0.188 10
    人均GDP 0.163 0.210 0.295 9
    工业用电量 −0.200 −0.137 −0.104 10
    城市绿化覆盖率 −0.540 −0.530 −0.515 10
    AICc 49.500
    R2 0.813
    调整R2 0.404
    下载: 导出CSV

    表  3  2015—2020年临汾市和大同市PM2.5、O3浓度与气象因子的Pearson相关系数

    Table  3.   Pearson correlation coefficient between PM2.5, O3 and meteorological factors in Linfen City and Datong City from 2015 to 2020

    城市气象因子Pearson相关系数
    PM2.5浓度O3浓度
    临汾市 风速 −0.338 9*** 0.170 8***
    平均气温 −0.486 5*** 0.744 5***
    降水量 −0.157 5*** −0.048 3
    平均相对湿度 0.050 2 −0.102 1***
    大同市 风速 −0.335 8*** 0.006 9
    平均气温 −0.312 6*** 0.779 8***
    降水量 −0.163 1*** 0.119 5***
    平均相对湿度 0.074 0** 0.050 7
    注:**表示P<0.002,***表示P<0.001.
    下载: 导出CSV
  • [1] BAI X X,TIAN H Z,LIU X Y,et al.Spatial-temporal variation characteristics of air pollution and apportionment of contributions by different sources in Shanxi Province of China[J].Atmospheric Environment,2021,244:117926. doi: 10.1016/j.atmosenv.2020.117926
    [2] ZHANG L C,AN J,LIU M Y,et al.Spatiotemporal variations and influencing factors of PM2.5 concentrations in Beijing,China[J].Environmental Pollution,2020,262:114276. doi: 10.1016/j.envpol.2020.114276
    [3] MAJI K J,SARKAR C.Spatio-temporal variations and trends of major air pollutants in China during 2015-2018[J].Environmental Science and Pollution Research,2020,27(27):33792-33808. doi: 10.1007/s11356-020-09646-8
    [4] CHEN J D,WANG B,HUANG S,et al.The influence of increased population density in China on air pollution[J].Science of the Total Environment,2020,735:139456. doi: 10.1016/j.scitotenv.2020.139456
    [5] HAN L J,ZHOU W Q,LI W F,et al.Impact of urbanization level on urban air quality:a case of fine particles (PM2.5) in Chinese cities[J].Environmental Pollution,2014,194:163-170. doi: 10.1016/j.envpol.2014.07.022
    [6] WANG S G,CHENG S Q,QI X H.Effect of urban greening on incremental PM2.5 concentration during peak hours[J].Frontiers in Public Health,2020,8:551300. doi: 10.3389/fpubh.2020.551300
    [7] XIE J L,SUN T L,LIU C F,et al.Quantitative evaluation of impacts of the steadiness and duration of urban surface wind patterns on air quality[J].Science of the Total Environment,2022,850:157957. doi: 10.1016/j.scitotenv.2022.157957
    [8] IKRAM M,YAN Z J,LIU Y,et al.Assessing the possible impacts of temperature change on air quality and public health in Beijing,2008-2012[J].Natural Hazards,2016,84(1):153-165.
    [9] RAVINDRA K,SINGH T,BISWAL A,et al.Impact of COVID-19 lockdown on ambient air quality in megacities of India and implication for air pollution control strategies[J].Environmental Science and Pollution Research ,2021,28(17):21621-21632. doi: 10.1007/s11356-020-11808-7
    [10] HU W Y,ZHAO T L,BAI Y Q,et al.Importance of regional PM2.5 transport and precipitation washout in heavy air pollution in the Twain-Hu Basin over Central China:observational analysis and WRF-Chem simulation[J].Science of the Total Environment,2021,758:143710. doi: 10.1016/j.scitotenv.2020.143710
    [11] FANG C L,LIU H M,LI G D,et al.Estimating the impact of urbanization on air quality in China using spatial regression models[J].Sustainability,2015,7(11):15570-15592. doi: 10.3390/su71115570
    [12] FOTHERINGHAM A S,YUE H,LI Z Q.Examining the influences of air quality in China´s cities using multi-scale geographically weighted regression[J].Transactions in GIS,2019,23(6):1444-1464. doi: 10.1111/tgis.12580
    [13] 王劲峰,徐成东.地理探测器:原理与展望[J].地理学报,2017,72(1):116-134. doi: 10.11821/dlxb201701010

    WANG J F,XU C D.Geodetector:principle and prospective[J].Acta Geographica Sinica,2017,72(1):116-134. doi: 10.11821/dlxb201701010
    [14] TORRENCE C,COMPO G P.A practical guide to wavelet analysis[J].Bulletin of the American Meteorological Society,1998,79(1):61-78. doi: 10.1175/1520-0477(1998)079<0061:APGTWA>2.0.CO;2
    [15] TAN S J,XIE D T,NI C S,et al.Spatiotemporal characteristics of air pollution in Chengdu-Chongqing urban agglomeration (CCUA) in Southwest,China:2015-2021[J].Journal of Environmental Management,2023,325:116503. doi: 10.1016/j.jenvman.2022.116503
    [16] 生态环境部.2016—2020年中国生态环境质量报告[M].北京:中国环境出版集团,2022:43-75.
    [17] 李瑞金,郝乾龙,刘洋,等.山西四城市大气污染特征及PM2.5传输规律研究[J].山西大学学报(自然科学版),2021,44(5):1031-1044.

    LI R J,HAO Q L,LIU Y,et al.Study on air pollution characteristics and PM2.5 transmission law in four cities of Shanxi Province[J].Journal of Shanxi University (Natural Science Edition),2021,44(5):1031-1044.
    [18] 焦姣,罗锦洪,杨锦锦,等.山西省城市地区近年来环境空气臭氧污染特征及来源解析[J].环境科学研究,2022,35(3):731-739.

    JIAO J,LUO J H,YANG J J,et al.Pollution characteristics and source apportionment of ground-level ozone in Shanxi urban region in recent years[J].Research of Environmental Sciences,2022,35(3):731-739.
    [19] FENG Y Y,NING M,LEI Y,et al.Defending blue sky in China:effectiveness of the ‘Air Pollution Prevention and Control Action Plan’ on air quality improvements from 2013 to 2017[J].Journal of Environmental Management,2019,252:109603. doi: 10.1016/j.jenvman.2019.109603
    [20] ZHAI S X,JACOB D J,WANG X A,et al.Fine particulate matter (PM2.5) trends in China,2013-2018:separating contributions from anthropogenic emissions and meteorology[J].Atmospheric Chemistry and Physics,2019,19(16):11031-11041. doi: 10.5194/acp-19-11031-2019
    [21] 李慧,王淑兰,张文杰,等.京津冀及周边地区“2+26”城市空气质量特征及其影响因素[J].环境科学研究,2021,34(1):172-184. doi: 10.13198/j.issn.1001-6929.2020.12.26

    LI H,WANG S L,ZHANG W J,et al.Characteristics and influencing factors of urban air quality in Beijing-Tianjin-Hebei and its surrounding areas (‘2+26’ cities)[J].Research of Environmental Sciences,2021,34(1):172-184. doi: 10.13198/j.issn.1001-6929.2020.12.26
    [22] 李慧,王涵,严沁,等.汾渭平原秋冬季PM2.5化学组分特征及其来源[J].环境科学研究,2023,36(3):449-459.

    LI H,WANG H,YAN Q,et al.Chemical composition characteristics and source apportionment of PM2.5 in the Fenwei Plain in autumn and winter[J].Research of Environmental Sciences,2023,36(3):449-459.
    [23] 张可可.基于长短时间序列分析的山西省大气PM2.5污染特征及影响因素研究[D].北京:华北电力大学,2022.
    [24] 山西省统计局.山西统计年鉴 2021[M].北京:中国统计出版社,2021.
    [25] LU B B,HU Y G,YANG D Y,et al.GWmodelS:a software for geographically weighted models[J].SoftwareX,2023,21:101291.
    [26] 卢宾宾,葛咏,秦昆,等.地理加权回归分析技术综述[J].武汉大学学报(信息科学版),2020,45(9):1356-1366.

    LU B B,GE Y,QIN K,et al.A review on geographically weighted regression[J].Geomatics and Information Science of Wuhan University,2020,45(9):1356-1366.
    [27] BRUNSDON C,FOTHERINGHAM A S,CHARLTON M E.Geographically weighted regression:a method for exploring spatial nonstationarity[J].Geographical Analysis,2010,28(4):281-298. doi: 10.1111/j.1538-4632.1996.tb00936.x
    [28] 覃文忠.地理加权回归基本理论与应用研究[D].上海:同济大学,2007:25-84.
    [29] YU H C,FOTHERINGHAM A S,LI Z Q,et al.Inference in multiscale geographically weighted regression[J].Geographical Analysis,2020,52(1):87-106. doi: 10.1111/gean.12189
    [30] FOTHERINGHAM A S,YANG W B,KANG W.Multiscale geographically weighted regression (MGWR)[J].Annals of the American Association of Geographers,2017,107(6):1247-1265. doi: 10.1080/24694452.2017.1352480
    [31] OSHAN T,LI Z Q,KANG W,et al.MGWR:a python implementation of multiscale geographically weighted regression for investigating process spatial heterogeneity and scale[J].ISPRS International Journal of Geo-Information,2019,8(6):269. doi: 10.3390/ijgi8060269
    [32] CAZELLES B,CHAVEZ M,BERTEAUX D,et al.Wavelet analysis of ecological time series[J].Oecologia,2008,156(2):287-304. doi: 10.1007/s00442-008-0993-2
    [33] GRINSTED A,MOORE J C,JEVREJEVA S.Application of the cross wavelet transform and wavelet coherence to geophysical time series[J].Nonlinear Processes in Geophysics,2004,11(5/6):561-566. doi: 10.5194/npg-11-561-2004
    [34] 环境保护部,国家质量监督检验检疫总局.环境空气质量标准:GB 3095—2012[S].北京:中国环境科学出版社,2012.
    [35] 吕梁市生态环境局.吕梁市“十四五”生态环境保护规划[R].吕梁:吕梁市人民政府办公室,2022.
    [36] 2020年山西省生态环境状况公报[R].太原:山西省生态环境厅,2021:3-4.
    [37] LI J D,HAO X,LIAO H,et al.Winter particulate pollution severity in North China driven by atmospheric teleconnections[J].Nature Geoscience,2022,15(5):349-355. doi: 10.1038/s41561-022-00933-2
    [38] WANG X Y,ZHANG R H.How did air pollution change during the COVID-19 outbreak in China?[J].Bulletin of the American Meteorological Society,2020,101(10):E1645-E1652. doi: 10.1175/BAMS-D-20-0102.1
    [39] 刘俊生.擦亮绿色发展城市底色打造生态宜居美丽大同[N].大同日报,2021-08-18(3).
    [40] 新华网.红色预警下,为何临汾二氧化硫污染屡次“破千”?[EB/OL].北京:新华网,(2017-01-17)[2023-08-11].http://www.xinhuanet.com/politics/2017-01/17/c_1120330971.htm.
    [41] HAREL O.The estimation of R2 and adjusted R2 in incomplete data sets using multiple imputation[J].Journal of Applied Statistics,2009,36(10):1109-1118. doi: 10.1080/02664760802553000
    [42] SONG H X,YANG M H.Analysis on effectiveness of SO2 emission reduction in Shanxi,China by satellite remote sensing[J].Atmosphere,2014,5(4):830-846. doi: 10.3390/atmos5040830
    [43] KAUFMANN R K,DAVIDSDOTTIR B,GARNHAM S,et al.The determinants of atmospheric SO2 concentrations:reconsidering the environmental Kuznets curve[J].Ecological Economics,1998,25(2):209-220. doi: 10.1016/S0921-8009(97)00181-X
    [44] LIU D R,DENG Q L,REN Z G,et al.Variation trends and principal component analysis of nitrogen oxide emissions from motor vehicles in Wuhan City from 2012 to 2017[J].Science of the Total Environment,2020,704:134987. doi: 10.1016/j.scitotenv.2019.134987
    [45] 山西省生态环境厅.山西省第二次全国污染源普查公报[R].太原:山西省生态环境厅,2020.
    [46] MIAO Z,BALEŽENTIS T,SHAO S,et al.Energy use,industrial soot and vehicle exhaust pollution:China´s regional air pollution recognition,performance decomposition and governance[J].Energy Economics,2019,83:501-514. doi: 10.1016/j.eneco.2019.07.002
    [47] CHEN Z Y,CHEN D L,ZHAO C F,et al.Influence of meteorological conditions on PM2.5 concentrations across China:a review of methodology and mechanism[J].Environment International,2020,139:105558. doi: 10.1016/j.envint.2020.105558
    [48] ROMER P S,DUFFEY K C,WOOLDRIDGE P J,et al.Effects of temperature-dependent NOx emissions on continental ozone production[J].Atmospheric Chemistry and Physics,2018,18(4):2601-2614. doi: 10.5194/acp-18-2601-2018
    [49] WANG W J,PARRISH D D,WANG S W,et al.Long-term trend of ozone pollution in China during 2014-2020:distinct seasonal and spatial characteristics and ozone sensitivity[J].Atmospheric Chemistry and Physics,2022,22(13):8935-8949. doi: 10.5194/acp-22-8935-2022
    [50] 张峻溪.人为源减排和气候变化对中国地区细颗粒物与臭氧的影响[D].杭州:浙江大学,2022:12-14.
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  • 收稿日期:  2023-05-15
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