Volume 35 Issue 12
Dec.  2022
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QUAN Shu, LIU Miaohan, CHEN Boxuan, HUANG Yuehua, MA Qingxia, HAN Yan. Characteristics of Near-Surface O3 Pollution and Its Relationship with Meteorological Factors in Henan Province[J]. Research of Environmental Sciences, 2022, 35(12): 2666-2676. doi: 10.13198/j.issn.1001-6929.2022.09.30
Citation: QUAN Shu, LIU Miaohan, CHEN Boxuan, HUANG Yuehua, MA Qingxia, HAN Yan. Characteristics of Near-Surface O3 Pollution and Its Relationship with Meteorological Factors in Henan Province[J]. Research of Environmental Sciences, 2022, 35(12): 2666-2676. doi: 10.13198/j.issn.1001-6929.2022.09.30

Characteristics of Near-Surface O3 Pollution and Its Relationship with Meteorological Factors in Henan Province

doi: 10.13198/j.issn.1001-6929.2022.09.30
Funds:  National Natural Youth Science Foundation of China (No.42105071); Henan Key Laboratory of Integrated Air Pollution Control and Ecological Security, China (No.PAP202101); Applied Technology Research Fund Project of Key Laboratory of Meteorological Disaster Prevention and Mitigation in Kaifeng, China Meteorological Administration (No.BQK202103)
  • Received Date: 2022-05-16
  • Rev Recd Date: 2022-08-14
  • Meteorological factors have an important influence on ozone (O3) concentration. In order to explore the characteristics and causes of near-surface O3 pollution in Henan Province, based on the datasets of ambient air quality monitoring stations and national basic ground climate stations in Henan Province from 2014 to 2020, this study examined the spatiotemporal characteristics of O3 pollution in Henan Province and the relationship between O3 and precursors and meteorological factors, and the potential sources of O3 in Henan Province were also explored. The results showed that: (1) In terms of temporal characteristics, the annual average O3 concentration of the maximum daily 8 h average (O3-8 h) in Henan Province generally decreased from 2014 to 2020, showing an ‘M’ type temporal evolution. For seasonality of O3-8 h concentration, it was highest in summer and decreased sequentially in spring, autumn, and winter, while both O3-8 h concentration and the number of days exceeding the standard peaked in June. In terms of spatial characteristics, the O3 concentration was generally lower in northern than in southern China, and lower in western than in eastern China. The areas with high concentrations were concentrated in southern Henan Province. (2) The O3-8 h concentration was significantly negatively correlated with the precursor NO2 and CO concentrations. (3) From the perspective of meteorological factors, O3-8 h concentration was positively correlated with air temperature and negatively correlated with relative humidity, indicating that high temperature (≥26 ℃) and low humidity (≤40%) were favorable for the increasing of O3-8 h concentration. Affected by the prevailing northerly winds in autumn and winter, the O3-8 h concentration in Henan Province showed a spatial pattern of low values in the north and high values in the south in autumn and winter, and the prevailing southerly wind in summer was conducive to the formation and maintenance of O3 in Henan Province. (4) In the summer of 2019, the main source areas of O3 and precursors increased gradually and changed from both inside and outside the province to mainly outside the province. Affected by the boundary cities and topographic conditions, O3 in Henan Province accumulated locally in summer. The study shows that the near-surface O3 pollution in Henan Province has significant spatial and temporal distribution characteristics, the pollution degree is generally reduced. The precursors of O3 and meteorological factors (temperature, relative humidity, wind) have significant effects on O3, and O3 transport paths and potential sources change with time in summer.

     

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