Volume 36 Issue 5
May  2023
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Article Contents
JING Qi, SHENG Lifang, ZHANG Weihang, AN Xiadong. Characteristics of PM2.5 and O3 Pollution and Related Meteorological Impacts in ‘2+26’ Cities of Beijing-Tianjin-Hebei and Its Surrounding Areas from 2018 to 2021[J]. Research of Environmental Sciences, 2023, 36(5): 875-886. doi: 10.13198/j.issn.1001-6929.2023.02.03
Citation: JING Qi, SHENG Lifang, ZHANG Weihang, AN Xiadong. Characteristics of PM2.5 and O3 Pollution and Related Meteorological Impacts in ‘2+26’ Cities of Beijing-Tianjin-Hebei and Its Surrounding Areas from 2018 to 2021[J]. Research of Environmental Sciences, 2023, 36(5): 875-886. doi: 10.13198/j.issn.1001-6929.2023.02.03

Characteristics of PM2.5 and O3 Pollution and Related Meteorological Impacts in ‘2+26’ Cities of Beijing-Tianjin-Hebei and Its Surrounding Areas from 2018 to 2021

doi: 10.13198/j.issn.1001-6929.2023.02.03
Funds:  National Natural Science Foundation of China (No.42275191)
  • Received Date: 2022-11-17
  • Rev Recd Date: 2023-02-07
  • In order to understand the air quality in key polluted areas in China, fine particulate matter (PM2.5) and ozone (O3) were studied during the Three-Year Action Plan to Win the Blue Sky Defense from 2018 to 2020 and in 2021. Specifically, the characteristics of PM2.5 and O3 compound pollution were analyzed using hourly monitoring data of PM2.5 and O3 in the ‘2+26’ cities of Beijing-Tianjin-Hebei and its surrounding areas. In addition, the contributions of emission sources and meteorological factors to the long-term trend of PM2.5 and O3 concentrations were quantified based on the KZ filter method. The results showed that in recent years, the annual mean PM2.5 and the 90th quantile of maximum daily 8-hour average ozone (O3-8 h-90th) concentrations decreased in the ‘2+26’ cities. The annual mean values of PM2.5 concentration from 2018 to 2021 were 60, 57, 51 and 45 μg/m3, respectively. The higher concentration of annual mean PM2.5 appeared in southern Hebei, Henan and southern Shandong provinces; O3-8 h-90th concentrations were 198, 195, 179 and 171 μg/m3, respectively. In 2018, O3-8 h-90th concentration was higher in Baoding, Shijiazhuang, Liaocheng and Jincheng (greater than 210 μg/m3), while Taiyuan O3-8 h-90th concentration was higher (192 μg/m3) in 2021. Furthermore, the long-term trend of PM2.5 and O3-8 h (maximum daily 8-hour average ozone) concentrations were more significantly influenced by meteorology. The long-term component of PM2.5 concentration affected by meteorology showed no obvious trend from 2018 to 2020 and a downward trend in 2021, while the long-term component of PM2.5 concentration affected by emissions showed a decreasing trend from 2018 to 2020 and no significant trend in 2021. The long-term component of O3-8 h concentration affected by meteorology showed an upward trend from 2018 to 2020 and a downward trend in 2021, while the long-term component of O3-8 h concentration affected by emissions showed a downward trend in 2018 and had no obvious trend from 2019 to 2021. Moreover, temperature and relative humidity had the greatest effect on both the concentration of PM2.5 and O3-8 h among the 11 meteorological factors. When the temperature and relative humidity increased together, it was more conducive to the simultaneous increase of PM2.5 and O3-8 h. The research shows that PM2.5 and O3 pollution in the ‘2+26’ cities are significantly affected by meteorology, and the changes in temperature and relative humidity are important in determining the simultaneous increase of PM2.5 and O3-8 h concentrations.

     

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  • [1]
    ZHAO S P,YIN D Y,YU Y,et al.PM2.5 and O3 pollution during 2015-2019 over 367 Chinese cities:spatiotemporal variations,meteorological and topographical impacts[J].Environmental Pollution,2020,264:114694. doi: 10.1016/j.envpol.2020.114694
    [2]
    QU L L,LIU S J,MA L L,et al.Evaluating the meteorological normalized PM2.5 trend (2014-2019) in the ‘2+26’ region of China using an ensemble learning technique[J].Environmental Pollution,2020,266:115346. doi: 10.1016/j.envpol.2020.115346
    [3]
    ZHANG Z Z,WANG W X,CHENG M M,et al.The contribution of residential coal combustion to PM2.5 pollution over China's Beijing-Tianjin-Hebei Region in winter[J].Atmospheric Environment,2017,159:147-161. doi: 10.1016/j.atmosenv.2017.03.054
    [4]
    LONG X,TIE X X,CAO J J,et al.Impact of crop field burning and mountains on heavy haze in the North China Plain:a case study[J].Atmospheric Chemistry and Physics,2016,16(15):9675-9691. doi: 10.5194/acp-16-9675-2016
    [5]
    WU G X,TIAN W L,ZHANG L,et al.The Chinese Spring Festival impact on air quality in China:a critical review[J].International Journal of Environmental Research and Public Health,2022,19(15):9074. doi: 10.3390/ijerph19159074
    [6]
    孙峰,姚欢,刘保献,等.2013—2019年京津冀及周边地区PM2.5重污染特征[J].中国环境监测,2021,37(4):46-53.

    SUN F,YAO H,LIU B X,et al.Characteristics of PM2.5 heavy pollution in Beijing-Tianjin-Hebei and surrounding areas from 2013 to 2019[J].Environmental Monitoring in China,2021,37(4):46-53.
    [7]
    井元元,李宏宇,张婧,等.1961—2017年华北区域大气自净能力变化特征及其影响因素分析[J].热带气象学报,2021,37(2):233-244.

    JING Y Y,LI H Y,ZHANG J,et al.Analysis of characteristics and influencing factors of atmospheric self-purification capacity in North China during 1961-2017[J].Journal of Tropical Meteorology,2021,37(2):233-244.
    [8]
    JIN X P,CAI X H,YU M Y,et al.Diagnostic analysis of wintertime PM2.5 pollution in the North China Plain:the impacts of regional transport and atmospheric boundary layer variation[J].Atmospheric Environment,2020,224:117346. doi: 10.1016/j.atmosenv.2020.117346
    [9]
    ZHANG W H,LI W S,AN X D,et al.Numerical study of the amplification effects of cold-front passage on air pollution over the North China Plain[J].Science of the Total Environment,2022,833:155231. doi: 10.1016/j.scitotenv.2022.155231
    [10]
    DANG R J,LIAO H.Severe winter haze days in the Beijing-Tianjin-Hebei Region from 1985 to 2017 and the roles of anthropogenic emissions and meteorology[J].Atmospheric Chemistry and Physics,2019,19(16):10801-10816. doi: 10.5194/acp-19-10801-2019
    [11]
    ZHANG X Y,XU X D,DING Y H,et al.The impact of meteorological changes from 2013 to 2017 on PM2.5 mass reduction in key regions in China[J].Science China:Earth Sciencess,2019,62(12):1885-1902. doi: 10.1007/s11430-019-9343-3
    [12]
    李慧,王淑兰,张文杰,等.京津冀及周边地区“2+26”城市空气质量特征及其影响因素[J].环境科学研究,2021,34(1):172-184. doi: 10.13198/j.issn.1001-6929.2020.12.26

    LI H,WANG S L,ZHANG W J,et al.Characteristics and influencing factors of urban air quality in Beijing-Tianjin-Hebei and its surrounding areas (‘2+26’ cities)[J].Research of Environmental Sciences,2021,34(1):172-184. doi: 10.13198/j.issn.1001-6929.2020.12.26
    [13]
    姜华,高健,李红,等.我国大气污染协同防控理论框架初探[J].环境科学研究,2022,35(3):601-610.

    JIANG H,GAO J,LI H,et al.Preliminary research on theoretical framework of cooperative control of air pollution in China[J].Research of Environmental Sciences,2022,35(3):601-610.
    [14]
    WEI J,LI Z Q,LI K,et al.Full-coverage mapping and spatiotemporal variations of ground-level ozone (O3) pollution from 2013 to 2020 across China[J].Remote Sensing of Environment,2022,270:112775. doi: 10.1016/j.rse.2021.112775
    [15]
    LI C L,LIU Y F,CHENG B F,et al.A comprehensive investigation on volatile organic compounds (VOCs) in 2018 in Beijing,China:characteristics,sources and behaviours in response to O3 formation[J].Science of the Total Environment,2022,806:150247. doi: 10.1016/j.scitotenv.2021.150247
    [16]
    DANG R J,LIAO H,FU Y.Quantifying the anthropogenic and meteorological influences on summertime surface ozone in China over 2012-2017[J].Science of the Total Environment,2021,754:142394. doi: 10.1016/j.scitotenv.2020.142394
    [17]
    GAO J,ZHANG J,LI H,et al.Comparative study of volatile organic compounds in ambient air using observed mixing ratios and initial mixing ratios taking chemical loss into account:a case study in a typical urban area in Beijing[J].Science of the Total Environment,2018,628/629:791-804. doi: 10.1016/j.scitotenv.2018.01.175
    [18]
    MA P F,MAO H Q,ZHANG J H,et al.Satellite monitoring of stratospheric ozone intrusion exceptional events:a typical case of China in 2019[J].Atmospheric Pollution Research,2022,13(2):101297. doi: 10.1016/j.apr.2021.101297
    [19]
    ZHANG Y J,ZHAO Y C,LI J,et al.Modeling ozone source apportionment and performing sensitivity analysis in summer on the North China plain[J].Atmosphere,2020,11(9):992. doi: 10.3390/atmos11090992
    [20]
    花丛,江琪,迟茜元,等.我国中东部地区2015—2020年夏半年PM2.5和臭氧复合污染气象特征分析[J].环境科学研究,2022,35(3):650-658.

    HUA C,JIANG Q,CHI X Y,et al.Meteorological characteristics of PM2.5-O3 air combined pollution in central and eastern China in the summer half years of 2015-2020[J].Research of Environmental Sciences,2022,35(3):650-658.
    [21]
    GONG S L,LIU Y L,HE J J,et al.Multi-scale analysis of the impacts of meteorology and emissions on PM2.5 and O3 trends at various regions in China from 2013 to 2020 1:synoptic circulation patterns and pollution[J].Science of the Total Environment,2022,815:152770. doi: 10.1016/j.scitotenv.2021.152770
    [22]
    ZHOU L H,ZHANG J,LU T W,et al.Pollution patterns and their meteorological analysis all over China[J].Atmospheric Environment,2021,246:118108. doi: 10.1016/j.atmosenv.2020.118108
    [23]
    YANG Z,YANG J,LI M M,et al.Nonlinear and lagged meteorological effects on daily levels of ambient PM2.5 and O3:evidence from 284 Chinese cities[J].Journal of Cleaner Production,2021,278:123931. doi: 10.1016/j.jclepro.2020.123931
    [24]
    GONG S L,ZHANG L,LIU C,et al.Multi-scale analysis of the impacts of meteorology and emissions on PM2.5 and O3 trends at various regions in China from 2013 to 2020 2.key weather elements and emissions[J].Science of the Total Environment,2022,824:153847. doi: 10.1016/j.scitotenv.2022.153847
    [25]
    DU H Y,LI J,WANG Z F,et al.Assessment of the effect of meteorological and emission variations on winter PM2.5 over the North China Plain in the three-year action plan against air pollution in 2018-2020[J].Atmospheric Research,2022,280:106395. doi: 10.1016/j.atmosres.2022.106395
    [26]
    WANG P F,GUO H,HU J L,et al.Responses of PM2.5 and O3 concentrations to changes of meteorology and emissions in China[J].Science of the Total Environment,2019,662:297-306. doi: 10.1016/j.scitotenv.2019.01.227
    [27]
    CHENG N L,CHENG B F,LI S S,et al.Effects of meteorology and emission reduction measures on air pollution in Beijing during heating seasons[J].Atmospheric Pollution Research,2019,10(3):971-979. doi: 10.1016/j.apr.2019.01.005
    [28]
    ESKRIDGE R E,KU J Y,RAO S T,et al.Separating different scales of motion in time series of meteorological variables[J].Bulletin of the American Meteorological Society,1997,78(7):1473-1483. doi: 10.1175/1520-0477(1997)078<1473:SDSOMI>2.0.CO;2
    [29]
    FANG C S,QIU J X,LI J,et al.Analysis of the meteorological impact on PM2.5 pollution in Changchun based on KZ filter and WRF-CMAQ[J].Atmospheric Environment,2022,271:118924. doi: 10.1016/j.atmosenv.2021.118924
    [30]
    GAO S,BAI Z P,LIANG S,et al.Simulation of surface ozone over Hebei Province,China using Kolmogorov-Zurbenko and artificial neural network (KZ-ANN) combined model[J].Atmospheric Environment,2021,261:118599. doi: 10.1016/j.atmosenv.2021.118599
    [31]
    RAO S T,ZURBENKO I G.Detecting and tracking changes in ozone air quality[J].Journal of the Air & Waste Management Association,1994,44(9):1089-1092.
    [32]
    SUN X Y,ZHAO T L,BAI Y Q,et al.Meteorology impact on PM2.5 change over a receptor region in the regional transport of air pollutants:observational study of recent emission reductions in Central China[J].Atmospheric Chemistry and Physics,2022,22(5):3579-3593. doi: 10.5194/acp-22-3579-2022
    [33]
    WISE E K,COMRIE A C.Extending the Kolmogorov-Zurbenko filter:application to ozone,particulate matter,and meteorological trends[J].Journal of the Air & Waste Management Association,2005,55(8):1208-1216.
    [34]
    张运江,雷若媛,崔世杰,等.2015—2020年我国主要城市PM2.5和O3污染时空变化趋势和影响因素[J].科学通报,2022,67(18):2029-2042.

    ZHANG Y J,LEI R Y,CUI S J,et al.Spatiotemporal trends and impact factors of PM2.5 and O3 pollution in major cities in China during 2015-2020[J].Chinese Science Bulletin,2022,67(18):2029-2042.
    [35]
    MILANCHUS M L,RAO S T,ZURBENKO I G.Evaluating the effectiveness of ozone management efforts in the presence of meteorological variability[J].Journal of the Air & Waste Management Association,1998,48(3):201-215.
    [36]
    彭玏.京津冀城市大气污染传输通道区2000—2015年PM2.5时空格局研究[D].北京:北京林业大学,2019:8-10.
    [37]
    WENG X,FORSTER G L,NOWACK P.A machine learning approach to quantify meteorological drivers of ozone pollution in China from 2015 to 2019[J].Atmospheric Chemistry and Physics,2022,22(12):8385-8402. doi: 10.5194/acp-22-8385-2022
    [38]
    GU R D,LI C F,LI D D,et al.The impact of rationalization and upgrading of industrial structure on carbon emissions in the Beijing-Tianjin-Hebei urban agglomeration[J].International Journal of Environmental Research and Public Health,2022,19(13):7997. doi: 10.3390/ijerph19137997
    [39]
    CHEN Y C,LEI T C,YAO S,et al.PM2.5 prediction model based on combinational Hammerstein recurrent neural networks[J].Mathematics,2020,8(12):2178. doi: 10.3390/math8122178
    [40]
    YU P,NIAN D,QIAO P J,et al.Memory behaviors of air pollutions and their spatial patterns in China[J].Frontiers in Physics,2022,10:875357. doi: 10.3389/fphy.2022.875357
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