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我国PM2.5与臭氧污染协同控制策略研究

李红 彭良 毕方 李陵 鲍捷萌 李俊玲 张浩 柴发合

李红, 彭良, 毕方, 李陵, 鲍捷萌, 李俊玲, 张浩, 柴发合. 我国PM2.5与臭氧污染协同控制策略研究[J]. 环境科学研究, 2019, 32(10): 1763-1778. doi: 10.13198/j.issn.1001-6929.2019.09.18
引用本文: 李红, 彭良, 毕方, 李陵, 鲍捷萌, 李俊玲, 张浩, 柴发合. 我国PM2.5与臭氧污染协同控制策略研究[J]. 环境科学研究, 2019, 32(10): 1763-1778. doi: 10.13198/j.issn.1001-6929.2019.09.18
LI Hong, PENG Liang, BI Fang, LI Ling, BAO Jiemeng, LI Junling, ZHANG Hao, CHAI Fahe. Strategy of Coordinated Control of PM2.5 and Ozone in China[J]. Research of Environmental Sciences, 2019, 32(10): 1763-1778. doi: 10.13198/j.issn.1001-6929.2019.09.18
Citation: LI Hong, PENG Liang, BI Fang, LI Ling, BAO Jiemeng, LI Junling, ZHANG Hao, CHAI Fahe. Strategy of Coordinated Control of PM2.5 and Ozone in China[J]. Research of Environmental Sciences, 2019, 32(10): 1763-1778. doi: 10.13198/j.issn.1001-6929.2019.09.18

我国PM2.5与臭氧污染协同控制策略研究

doi: 10.13198/j.issn.1001-6929.2019.09.18
基金项目: 

北京市科委首都蓝天行动培育专项 Z181100005418015

详细信息
    作者简介:

    李红(1969-), 女, 湖北洪湖人, 研究员, 博士, 主要从事大气光化学机理与臭氧污染防治、有毒有害有机物环境影响研究, lihong@craes.org.cn

    通讯作者:

    柴发合(1955-), 男, 陕西大荔人, 研究员, 博导, 中国环境科学研究院大气领域首席科学家, 主要从事大气污染控制与环境管理研究, chaifh@craes.org.cn

  • 中图分类号: X513

Strategy of Coordinated Control of PM2.5 and Ozone in China

Funds: 

Capital Blue Sky Action Training Project from Beijing Municipal Science & Technology Commission, China Z181100005418015

  • 摘要: 近年来,我国大气污染格局发生了深刻变化,PM2.5与臭氧(O3)成为影响我国城市和区域空气质量的主要空气污染物,二者协同控制已成为我国空气质量改善的焦点和打赢蓝天保卫战的关键.PM2.5与臭氧之间具有复杂的关联性,使得二者的协同控制具有复杂性与艰巨性.分析了PM2.5与臭氧成因的关联性及其相互影响,阐明了PM2.5与臭氧污染协同控制所涉及的重要科学问题,并在此基础上研究了目前我国PM2.5与臭氧的污染形势及二者的关联性,梳理了我国自2013年以来在PM2.5与臭氧污染控制中已采取的重要举措,论述了目前我国PM2.5与臭氧协同控制在科学与管理上所面临的挑战.结合对国外成功经验的分析,提出推进我国PM2.5与臭氧污染协同控制工作的相关建议:①加快监测能力建设,完善管理体系;②强化科技支撑,提高PM2.5与臭氧污染控制精准性;③加快构建VOCs与NOx治理技术体系;④加大VOCs与NOx的协同减排力度,保障减排方案落实到位.

     

  • 图  1  对流层中二次气溶胶和臭氧生成机制示意图[23-24, 37, 40-42]

    注:hν表示光照.虚线箭头表示复杂多步反应.加粗文字表示生成的二次产物. g表示气态,l表示液态.

    Figure  1.  A schematic picture of the forming mechanisms of secondary aerosol and ozone in the troposphere[23-24, 37, 40-42]

    图  2  2015—2018年338个城市ρ(PM2.5)年均值和ρ(O3)年评价值不同数值区间的城市数量占比

    Figure  2.  The ratio of the number of cities with different mass concentration ranges of PM2.5 and ozone in 338 cities from 2015 to 2018

    图  3  2015年与2018年重点区域ρ(PM2.5)年均值变化情况

    注:各城市PM2.5和臭氧监测数据来源于中国环境监测总站的全国城市空气质量实时发布平台(http://106.37.208.233:20035).京津冀及周边地区(“2+26”城市)城市包含北京市,天津市,河北省的石家庄市、唐山市、邯郸市、邢台市、保定市、沧州市、廊坊市、衡水市和雄安新区,山西省的太原市、阳泉市、长治市和晋城市,山东省的济南市、淄博市、济宁市、德州市、聊城市、滨州市和菏泽市,河南省的郑州市、开封市、安阳市、鹤壁市、新乡市、焦作市和濮阳市.珠三角地区城市包含广州市、深圳市、佛山市、东莞市、中山市、惠州市、珠海市、江门市、肇庆市.长三角地区城市包含上海市、江苏省、浙江省和安徽省.汾渭平原包含山西省的晋中市、运城市、临汾市、吕梁市,河南省的洛阳市、三门峡市,陕西省的西安市、铜川市、宝鸡市、咸阳市、渭南市以及杨凌示范区.成渝城市群包括重庆市, 四川省的成都市、自贡市、泸州市、德阳市、绵阳市、遂宁市、内江市、乐山市、南充市、眉山市、宜宾市、广安市、达州市、雅安市、资阳市. 338个城市中的其他城市(略).下同.

    Figure  3.  The annual variation of PM2.5 mass concentration in key regions between 2015 and 2018

    图  4  2015年与2018年重点区域ρ(O3)年评价值变化情况

    Figure  4.  The annual variation of the 90th of O3-8 h max mass concentration in key regions between 2015 and 2018

    图  5  2013—2017年国家环境空气背景站点ρ(O3)年评价值的年际变化

    Figure  5.  The annual variation of the 90th of O3-8 h max mass concentration at national environmental air quality monitoring background station from 2013 to 2017

    图  6  2018年重点区域地面ρ(O3)日最大8 h平均值随ρ(PM2.5)日均值变化的情况

    Figure  6.  The variation of the 90th of O3-8 h max mass concentration with daily mean PM2.5 in key regions in 2018

  • [1] Clean Air Asia.Breakthroughs: China's path to clean air 2013-2017[R/OL].Beijing: Clean Air Asia, 2018[2019-07-20].http://www.allaboutair.cn/a/reports/2018/1227/527.html.
    [2] ZHENG B, TONG D, LI M, et al.Trends in China's anthropogenic emissions since 2010 as the consequence of clean air actions[J].Atmospheric Chemistry and Physics, 2018, 18(19):14095-14111. doi: 10.5194/acp-18-14095-2018
    [3] 生态环境部.中国空气质量改善报告(2013-2018年)[R].北京: 生态环境部, 2019: 1-5.
    [4] WANG Pengfei, GUO Hao, HU Jianlin, et al.Responses of PM2.5 and O3 concentrations to changes of meteorology and emissions in China[J].Science of the Total Environment, 2019, 662:297-306. doi: 10.1016/j.scitotenv.2019.01.227
    [5] LI Ke, JACOB D J, LIAO Hong, et al.Anthropogenic drivers of 2013-2017 trends in summer surface ozone in China[J].Proceedings of the National Academy of Sciences of the United States of America, 2019, 116(2):422-427. doi: 10.1073/pnas.1812168116
    [6] LYU Xiaopu, WANG Nan, GUO Hai, et al.Causes of a continuous summertime O3 pollution event in Jinan, a central city in the North China Plain[J].Atmospheric Chemistry and Physics, 2019, 19(5):3025-3042. doi: 10.5194/acp-19-3025-2019
    [7] QU Yawei, WANG Tijian, CAI Yanfeng, et al.Influence of atmospheric particulate matter on ozone in Nanjing, China:observational study and mechanistic analysis[J].Advances in Atmospheric Sciences, 2018, 35(11):1381-1395. doi: 10.1007/s00376-018-8027-4
    [8] TAN Zhaofeng, LU Keding, JIANG Meiqing, et al.Exploring ozone pollution in Chengdu, southwestern China:a case study from radical chemistry to O3-VOC-NOx sensitivity[J].Science of the Total Environment, 2018, 636:775-786. doi: 10.1016/j.scitotenv.2018.04.286
    [9] Anon.Cleaner air for China[J].Nature Geoscience, 2019, 12(7):497. doi: 10.1038/s41561-019-0406-7
    [10] AN Zhisheng, HUANG Rujin, ZHANG Renyi, et al.Severe haze in northern China:asynergy of anthropogenic emissions and atmospheric processes[J].Proceedings of the National Academy of Sciences of the United States of America, 2019, 116(18):8657-8666. doi: 10.1073/pnas.1900125116
    [11] HU Jianlin, WU Li, ZHEGN Bo, et al.Source contributions and regional transport of primary particulate matter in China[J].Environmental Pollution, 2015, 207:31-34. doi: 10.1016/j.envpol.2015.08.037
    [12] 柴发合.中国未来三年大气污染治理形势预判与对策分析[J].中国环境监察, 2019(1):29-31. http://www.cnki.com.cn/Article/CJFDTotal-HJJC201901010.htm

    CHAI Fahe.Analysis of control situation prediction and countermeasures of China's air pollution in the next three years[J].China Environmental Monitoring, 2019(1):29-31. http://www.cnki.com.cn/Article/CJFDTotal-HJJC201901010.htm
    [13] DING A J, FU C B, YANG X Q, et al.Ozone and fine particle in the western Yangtze River Delta:an overview of 1 yr data at the SORPES station[J].Atmospheric Chemistry and Physics, 2013, 13(11):5813-5830. doi: 10.5194/acp-13-5813-2013
    [14] 国务院.国务院关于印发打赢蓝天保卫战三年行动计划的通知[R].北京: 国务院, 2018: 1-2.
    [15] XING Jia, WANG Jiandong, MATHUR R, et al.Impacts of aerosol direct effects on tropospheric ozone through changes in atmospheric dynamics and photolysis rates[J].Atmospheric Chemistry and Physics, 2017, 17(16):9869-9883. doi: 10.5194/acp-17-9869-2017
    [16] XU Jun, ZHANG Yuanhang, ZHENG Shaoqing.Aerosol effects on ozone concentrations in Beijing:a model sensitivity study[J].Journal of Environmetal Sciences, 2012, 24(4):645-656. doi: 10.1016/S1001-0742(11)60811-5
    [17] WANG Shaojian, ZHOU Chunshan, WANG Zhenbo, et al.The characteristics and drivers of fine particulate matter (PM2.5) distribution in China[J].Journal of Cleaner Production, 2017, 142(4):1800-1809. http://www.sciencedirect.com/science/article/pii/S0959652616319497
    [18] DUAN Jingchun, TAN Jihua, HAO Jiming, et al.Size distribution, characteristics and sources of heavy metals in haze episod in Beijing[J].Journal of Environmental Science, 2014, 6(1):189-196. http://d.old.wanfangdata.com.cn/Periodical/jes-e201401022
    [19] 杜祯宇, 殷惠民, 张烃.细颗粒物与臭氧协同控制的方法和必要性[J].世界环境, 2018(1):19-20. http://d.old.wanfangdata.com.cn/Periodical/sjhj201801007

    DU Zhenyu, YIN Huimin, ZHANG Ting.The methods and necessity of coordinated control of fine particulate matter and ozone[J].World Environment, 2018(1):19-20. http://d.old.wanfangdata.com.cn/Periodical/sjhj201801007
    [20] ZHANG Renyi, WANG Gehui, GUO Song, et al.Formation of urban fine particulate matter[J].Chemical Reviews, 2015, 115(10):3803-3855. doi: 10.1021/acs.chemrev.5b00067
    [21] FUZZI S, BALTENSPERGER U, CARSLAW K, et al.Particulate matter, air quality and climate:lessons learned and future needs[J].Atmospheric Chemistry and Physics, 2015, 15(14):8217-8299. doi: 10.5194/acp-15-8217-2015
    [22] WANG Gehui, ZHANG Renyi, GOMEZ M E, et al.Persistent sulfate formation from London Fog to Chinese haze[J].Proceedings of the National Academy of Sciences of the United States of America, 2016, 113(48):13630-13635. doi: 10.1073/pnas.1616540113
    [23] CHENG Yafeng, ZHENG Guangjie, WEI Chao, et al.Reactive nitrogen chemistry in aerosol water as a source of sulfate during haze events in China[J].Science Advances, 2016.doi: 10.1126/sciadv.1601530.
    [24] SARWAR G, FAHEY K, KWORK R, et al.Potential impacts of two SO2 oxidation pathways on regional sulfate concentrations:aqueous-phase oxidation by NO2 and gas-phase oxidation by stabilized criegee intermediates[J].Atmospheric Environment, 2013, 68:186-197. doi: 10.1016/j.atmosenv.2012.11.036
    [25] CHEN L, LIU R M, HUANG Q, et al.An integrated simulation-monitoring framework for nitrogen assessment:a case study in the Baixi watershed, China[J].Procedia Environmental Sciences, 2012, 13:1076-1090. doi: 10.1016/j.proenv.2012.01.101
    [26] HUSAIN L, RATTIGAN O V, DUTKIEWICZ V, et al. Case studies of the SO2+H2O2 reaction in clouds[J]. Journal of Geophysical Research Atmospheres, 2000, 105(D8):9831-9841. doi: 10.1029/1999JD901177
    [27] ALEXANDER B.Quantifying global atmospheric sulfate formation pathways utilizing observations and modeling of the oxygen isotopic composition (Δ17O) of sulfate aerosol (Invited)[C]//American Geophysical Union.AGU Fall Meeting Abstracts.Seattle: American Geophysical Union, 2010: A44A-05.
    [28] PATHAK R K, WANG Tao, LEE K F, et al.Characteristics of summertime PM2.5 organic and elemental carbon in four major Chinese cities:implications of high acidity for water-soluble organic carbon (WSOC)[J].Atmospheric Environment, 2011, 45(2):318-325. doi: 10.1016/j.atmosenv.2010.10.021
    [29] GRIFFITH S M, HUANG X H H, LOUIE P K K, et al.Characterizing the thermodynamic and chemical composition factors controlling PM2.5 nitrate:insights gained from two years of online measurements in Hong Kong[J].Atmospheric Environment, 2015, 122:864-875. doi: 10.1016/j.atmosenv.2015.02.009
    [30] WANG Xinfeng, WANG Wenxing, YANG Lingxiao, et al.The secondary formation of inorganic aerosols in the droplet mode through heterogeneous aqueous reactions under haze conditions[J].Atmospheric Environment, 2012, 63:68-76. doi: 10.1016/j.atmosenv.2012.09.029
    [31] 谢绍东, 田晓雪.挥发性和半挥发性有机物向二次有机气溶胶转化的机制[J].化学进展, 2010, 22(4):727-733. http://www.wanfangdata.com.cn/details/detail.do?_type=perio&id=hxjz201004020

    XIE Shaodong, TIAN Xiaoxue.Formation mechanism of secondary organic aerosols from the reaction of volatile and semi-volatile compounds[J].Progress in Chemistry, 2010, 22(4):727-733. http://www.wanfangdata.com.cn/details/detail.do?_type=perio&id=hxjz201004020
    [32] 方文政.大气氧化及光氧化挥发性有机物生成二次有机气溶胶的研究[D].合肥: 中国科学技术大学, 2012. http://cdmd.cnki.com.cn/Article/CDMD-10358-1012503730.htm
    [33] DANIELSEN E F.Stratospheric-tropospheric exchange based on radioactivity, ozone and potential vorticity[J].Journal of the Atmospheric Sciences, 1968, 25(3):502-518. doi: 10.1175/1520-0469(1968)025<0502:STEBOR>2.0.CO;2
    [34] CRUTZEN P A.Discussion of the chemistry of some minor constituents in the stratosphere and troposphere[J].Pure & Applied Geophysics, 1973, 106/107/108(1):1385-1399. doi: 10.1007/BF00881092
    [35] ALLEN S K, PLATTNER G K, NAUELS A, et al.Climate change 2013:the physical science basis.an overview of the working group 1 contribution to the fifth assessment report of the Intergovernmental Panel on Climate Change (IPCC)[J].Computational Geometry, 2007, 18(2):95-123. http://adsabs.harvard.edu/abs/2014EGUGA..16.3544A
    [36] MONKS P S, ARCHIBALD AT, COLETTE A, et al.Tropospheric ozone and its precursors from the urban to the global scale from air quality to short-lived climate forcer[J].Atmospheric Chemistry and Physics, 2015, 15(15):8889-8973. doi: 10.5194/acp-15-8889-2015
    [37] WANG Tao, XUE Likun, BRIMBLECOMBE P, et al.Ozone pollution in China:a review of concentrations, meteorological influences, chemical precursors, and effects[J].Science of the Total Environment, 2017, 575:1582-1596. doi: 10.1016/j.scitotenv.2016.10.081
    [38] POISSON N, KANAKIDOU M, BONSANG B, et al.The impact of natural non-methane hydrocarbon oxidation on the free radical and ozone budgets above a eucalyptus forest[J].Chemosphere, 2001, 3:353-366. http://www.sciencedirect.com/science/article/pii/S1465997201000162
    [39] ATKINSON R.Atmospheric chemistry of VOCs and NOx[J].Atmospheric Environment, 2000, 34:2063-2101. doi: 10.1016/S1352-2310(99)00460-4
    [40] LU Keding, GUO Song, TAN Zhaofeng, et al.Exploring atmospheric free-radical chemistry in China:the self-cleansing capacity and the formation of secondary air pollution[J].National Science Review, 2019, 6(3):579-594. doi: 10.1093/nsr/nwy073
    [41] XUE L K, WANG T, GAO J, et al.Ground-level ozone in four Chinese cities:precursors, regional transport and heterogeneous processes[J].Atmospheric Chemistry and Physics, 2014, 14(23):13175-13188. doi: 10.5194/acp-14-13175-2014
    [42] DAGAUT P.Kinetics of oxygen-containing organic compounds with hydroxyl radicals in the gas phase:a review for modeling combustion and atmospheric chemistry[J].Journal de Chimie Physique et de Physico-Chimie Biologique, 1989, 86:595-623. doi: 10.1051/jcp/1989860595
    [43] SASSEN K.Indirect climate forcing over the western US from Asian dust storms[J].Geophysical Research Letters, 2002.doi: 10.1029/2001gl014051.
    [44] KUMAR R, BARTH M C, MADRONICH S, et al.Effects of dust aerosols on tropospheric chemistry during a typical pre-monsoon season dust storm in northern India[J].Atmospheric Chemistry and Physics, 2014, 14(13):6813-6834. doi: 10.5194/acp-14-6813-2014
    [45] 邵平, 辛金元, 安俊琳, 等.长三角工业区夏季近地层臭氧和颗粒物污染相互关系研究[J].大气科学, 2017, 41(3):618-628. http://d.old.wanfangdata.com.cn/Periodical/daqikx201703014

    SHAO Ping, XIN Jinyuan, AN Junlin, et al.An analysis on the relationship between ground-level ozone and particulate matter in an industrial area in the Yangtze River Delta during summertime[J].Chinese Journal of Atmospheric Sciences, 2017, 41(3):618-628. http://d.old.wanfangdata.com.cn/Periodical/daqikx201703014
    [46] JIA Xing, MATHUR R, PLEIM J, et al.Air pollution and climate response to aerosol direct radiative effects:a modeling study of decadal trends across the northern hemisphere[J].Journal of Geophysical Research Atmospheres, 2015, 120(23):12221-12236. doi: 10.1002/2015JD023933/pdf
    [47] SAATHOFF H, NAUMANN K H, MOEHLER O, et al.Temperature dependence of yields of secondary organic aerosols from the ozonolysis of alpha-pinene and limonene[J].Atmospheric Chemistry and Physics, 2009, 9(5):1551-1577. doi: 10.5194/acp-9-1551-2009
    [48] LI J, WANG Z, WANG X, et al.Impacts of aerosols on summertime tropospheric photolysis frequencies and photochemistry over Central Eastern China[J].Atmospheric Environment, 2011, 45(10):1817-1829. doi: 10.1016/j.atmosenv.2011.01.016
    [49] YUAN Tianle, REMER L A, BIAN Huisheng, et al.Aerosol indirect effect on tropospheric ozone via lightning[J].Journal of Geophysical Research, 2012, 117:D18213. doi: 10.1029/2012JD017723/citedby
    [50] LOU Sijia, LIAO Hong, ZHU Bin.Impacts of aerosols on surface-layer ozone concentrations in China through heterogeneous reactions and changes in photolysis rates[J].Atmospheric Environment, 2014, 85:123-138. doi: 10.1016/j.atmosenv.2013.12.004
    [51] LI Jie, CHEN Xueshun, WANG Zifa, et al.Radiative and heterogeneous chemical effects of aerosols on ozone and inorganic aerosols over East Asia[J].Science of the Total Environment, 2018, 622/623:1327-1342. doi: 10.1016/j.scitotenv.2017.12.041
    [52] DU Huiyun, LI Jie, CHEN Xueshun, et al.Modeling of aerosol property evolution during winter haze episodes over a megacity cluster in northern China:roles of regional transport and heterogeneous reactions of SO2[J].Atmospheric Chemistry and Physics, 2019, 19(14):9351-9370. doi: 10.5194/acp-19-9351-2019
    [53] HUANG Rujin, ZHANG Yanlin, BOZZETTI C, et al.High secondary aerosol contribution to particulate pollution during haze events in China[J].Nature, 2014, 514(7521):218-222. doi: 10.1038/nature13774
    [54] LEE A K Y.Haze formation in China:importance of secondary aerosol[J].Journal of Environmental Science, 2015, 33:261-262. doi: 10.1016/j.jes.2015.06.002
    [55] 唐孝炎, 张远航, 邵敏.大气环境化学[M].2版.北京:高等教育出版社, 2006:101-121.
    [56] 李干杰.生态环境部部长李干杰就"打好污染防治攻坚战"答记者问[J].中国环境监察, 2019(S1):12-25.

    LI Ganjie.Minister of the Ministry of Eco-Environment, answered questions on 'Being a good fight against pollution prevention and control'[J].China Environmental Monitoring, 2019(S1):12-25.
    [57] AKIMOTO H, NAGASHIMA T, LI Jie, et al.Comparison of surface ozone simulation among selected regional models in MICS:Asia Ⅲ.effects of chemistry and vertical transport for the causes of difference[J].Atmospheric Chemistry and Physics, 2019, 19(1):603-615. doi: 10.5194/acp-19-603-2019
    [58] EHN M, THORNTON J A, KLEIST E, et al.A large source of low-volatility secondary organic aerosol[J].Nature, 2014, 506(7489):476-479. doi: 10.1038/nature13032
    [59] WANG Tao, THAM Y J, XUE Likun, et al.Observations of nitryl chloride and modeling its source and effect on ozone in the planetary boundary layer of southern China[J].Journal of Geophysical Research:Atmospheres, 2016, 121(5):2476-2489. doi: 10.1002/2015JD024556
    [60] 生态环境部.2018年中国生态环境状况公报[R].北京: 生态环境部, 2019: 1-15.
    [61] CHEN Hai, ZHUANG Bingliang, LIU Jane, et al.Characteristics of ozone and particles in the near-surface atmosphere in the urban area of the Yangtze River Delta, China[J].Atmospheric Chemistry and Physics, 2019, 19(7):4153-4175. doi: 10.5194/acp-19-4153-2019
    [62] CRISTOFANELLI P, BONASONI P.Background ozone in the southern Europe and Mediterranean area:influence of the transport processes[J].Environmental Pollution, 2009, 157(5):1399-1406. doi: 10.1016/j.envpol.2008.09.017
    [63] LI Jie, YANG Wenyi, WANG Zifa, et al.Modeling study of surface ozone source-receptor relationships in East Asia[J].Atmospheric Research, 2016, 167:77-88. doi: 10.1016/j.atmosres.2015.07.010
    [64] VERSTRAETEN W W, NEU J L, WILLIAMS J E, et al.Rapid increases in tropospheric ozone production and export from China[J].Nature Geoscience, 2015, 8(9):690-695. doi: 10.1038/ngeo2493
    [65] ZOU Y, DENG X J, ZHU D, et al.Characteristics of 1 year of observational data of VOCs, NOx and O3 at a suburban site in Guangzhou, China[J].Atmospheric Chemistry and Physics, 2015, 15(12):6625-6636. doi: 10.5194/acp-15-6625-2015
    [66] OU Jiamin, YUAN Zibing, ZHENG Junyu, et al.Ambient ozone control in a photochemically active region:short-term despiking or long-term attainment[J].Environmental Science & Technology, 2016, 50(11):5720-5728. doi: 10.1021/acs.est.6b00345
    [67] LI Qinyi, ZHANG Li, WANG Tao, et al.'New' reactive nitrogen chemistry reshapes the relationship of ozone to its precursors[J].Environmental Science & Technology, 2018, 52(5):2810-2818. http://europepmc.org/abstract/MED/29406712
    [68] ZHANG Li, LI Qinyi, WANG Tao, et al.Combined impacts of nitrous acid and nitryl chloride on lower-tropospheric ozone:new module development in WRF-Chem and application to China[J].Atmospheric Chemistry and Physics, 2017, 17(16):9733-9750. doi: 10.5194/acp-17-9733-2017
    [69] WANG Jing, ALLEN D J, PICKERING K E, et al.Impact of aerosol direct effect on East Asian air quality during the EAST-AIRE campaign[J].Journal of Geophysical Research:Atmospheres, 2016, 121(11):6534-6554. doi: 10.1002/2016JD025108
    [70] GUO Song, HU Min, ZAMORA M L, et al.Elucidating severe urban haze formation in China[J].Proceedings of the National Academy of Sciences of the United States of America, 2014, 111(49):17373-17378. doi: 10.1073/pnas.1419604111
    [71] 曹军骥.PM2.5与环境[M].北京:科学出版社, 2014:1-14.
    [72] 张华, 陈琪, 谢冰, 等.中国的PM2.5和对流层臭氧及污染物排放控制对策的综合分析[J].气候变化研究进展, 2014, 10(4):289-296. doi: 10.3969/j.issn.1673-1719.2014.04.010

    ZHANG Hua, CHEN Qi, XIE Bing, et al.PM2.5 and tropospheric ozone in China and pollution emission controlling integrated analyses[J].Advances in Climate Change Research, 2014, 10(4):289-296. doi: 10.3969/j.issn.1673-1719.2014.04.010
    [73] 张远航, 王金南.发达国家有哪些大气治理经验值得我们借鉴[N/OL].北京: 中国环境报, 2017-03-03[2019-07-20]. https://www.cenews.com.cn/news/201703/t20170303_823825.html.
    [74] 薛志钢, 郝吉明, 陈复, 等.国外大气污染控制经验[J].重庆环境科学, 2003, 25(11):159-161. doi: 10.3969/j.issn.1674-2842.2003.11.057
    [75] TABLER S K.EPA's program for establishing national emission standards for hazardous air pollutants[J].Journal of the Air Pollution Control Association, 1984, 34(5):532-536. doi: 10.1080/00022470.1984.10465771
    [76] 柴发合, 王晓, 罗宏, 等.美国与欧盟关于PM和臭氧的监管政策述评[J].环境工程技术学报, 2013, 3(1):46-52. doi: 10.3969/j.issn.1674-991X.2013.01.009

    CHAI Fahe, WANG Xiao, LUO Hong, et al.Review of supervision policies of USA and European Union on PM2.5 and O3[J].Journal of Environmental Engineering Technology, 2013, 3(1):46-52. doi: 10.3969/j.issn.1674-991X.2013.01.009
    [77] Department for Environment, Food & Rural Affairs.The air quality strategy for England, Scotland, Wales and Northern Ireland (Volume 1)[R/OL].London: The Stationery Office, 2007[2019-07-30].http://www.apis.ac.uk/overview/regulations/overview_UK_NAQS.htm.
    [78] European Environment Agency.Air pollutant emissions data viewer (LRTAP Convention)[EB/OL].Copenhagen: European Environment Agency Web, 2017-08-21[2019-07-30].http://www.eea.europa.eu/data-and-maps/data/data-viewers/air-emissions-viewer-lrtap.
    [79] 郑军, 袁钰.欧洲大气污染防治经验及对我国的启示[J].环境保护, 2017, 45(18):68-70. http://d.old.wanfangdata.com.cn/Periodical/hjbh201718015

    ZHENG Jun, YUAN Yu.Experience of air pollution preventon and control in europe and its enlightenment to China[J].Environmental Protection, 2017, 45(18):68-70. http://d.old.wanfangdata.com.cn/Periodical/hjbh201718015
    [80] SOLBERG S, DERWENT R G, HOV Y, et al.European abatement of surface ozone in a global perspective[J].AMBIO:A Journal of the Hunman Environment, 2005, 34(1):47-53. doi: 10.1579/0044-7447-34.1.47
    [81] 杜譞, 李宏涛.欧美经验对我国"十三五"大气污染防治战略的启示[J].中国环境管理, 2016, 8(5):57-62. http://www.wanfangdata.com.cn/details/detail.do?_type=perio&id=90727176504849544853484954

    DU Xuan, LI Hongtao.European and American experiences and its implications on air pollution control strategy in China during the 13th Five-Year Period[J].Chinese Journal of Environmental Management, 2016, 8(5):57-62. http://www.wanfangdata.com.cn/details/detail.do?_type=perio&id=90727176504849544853484954
    [82] 亚洲清洁空气中心.美国加州湾区臭氧管控经验[R/OL].北京: 亚洲清洁空气中心, 2016[2019-07-20]. http://allaboutair.cn/a/experience_intl//2016/0409/442.html.
    [83] CHEN Dan, LI Qinbin, STUTZ J, et al.WRF-Chem simulation of NOx and O3 in the L.A. basin during CalNex-2010[J].Atmospheric Environment, 2013, (81):421-432. http://www.sciencedirect.com/science/article/pii/S1352231013006845
    [84] United States Environmental Protection Agency.Ozone air quality, 1980-2018[EB/OL].Washington DC: US EPA, 2019-07-03[2019-07-30].https://www.epa.gov/air-trends/ozone-trends.
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  • 收稿日期:  2019-08-19
  • 修回日期:  2019-09-22
  • 刊出日期:  2019-10-25

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