留言板

尊敬的读者、作者、审稿人, 关于本刊的投稿、审稿、编辑和出版的任何问题, 您可以本页添加留言。我们将尽快给您答复。谢谢您的支持!

姓名
邮箱
手机号码
标题
留言内容
验证码

2015—2020年中国臭氧污染时空演化及其与厄尔尼诺-南方涛动的关系研究

杨艺科 王晓红 凌元锦 陆庆恒 秦靖蒿 李晓艺 于乐江

杨艺科, 王晓红, 凌元锦, 陆庆恒, 秦靖蒿, 李晓艺, 于乐江. 2015—2020年中国臭氧污染时空演化及其与厄尔尼诺-南方涛动的关系研究[J]. 环境科学研究, 2023, 36(5): 895-903. doi: 10.13198/j.issn.1001-6929.2023.03.03
引用本文: 杨艺科, 王晓红, 凌元锦, 陆庆恒, 秦靖蒿, 李晓艺, 于乐江. 2015—2020年中国臭氧污染时空演化及其与厄尔尼诺-南方涛动的关系研究[J]. 环境科学研究, 2023, 36(5): 895-903. doi: 10.13198/j.issn.1001-6929.2023.03.03
YANG Yike, WANG Xiaohong, LING Yuanjin, LU Qingheng, QIN Jinghao, LI Xiaoyi, YU Lejiang. Spatial-Temporal Evolution of Ozone Pollution and Its Relationship with El Niño-Southern Oscillation in China from 2015 to 2020[J]. Research of Environmental Sciences, 2023, 36(5): 895-903. doi: 10.13198/j.issn.1001-6929.2023.03.03
Citation: YANG Yike, WANG Xiaohong, LING Yuanjin, LU Qingheng, QIN Jinghao, LI Xiaoyi, YU Lejiang. Spatial-Temporal Evolution of Ozone Pollution and Its Relationship with El Niño-Southern Oscillation in China from 2015 to 2020[J]. Research of Environmental Sciences, 2023, 36(5): 895-903. doi: 10.13198/j.issn.1001-6929.2023.03.03

2015—2020年中国臭氧污染时空演化及其与厄尔尼诺-南方涛动的关系研究

doi: 10.13198/j.issn.1001-6929.2023.03.03
基金项目: 山东省自然科学基金项目(No.ZR2020MD016)
详细信息
    作者简介:

    杨艺科(1998-),男,河南许昌人,yangkepersonal@outlook.com

    通讯作者:

    王晓红(1981-),女,山东淄博人,副教授,博士,主要从事大气环境污染研究,28473356@qq.com

  • 中图分类号: X513

Spatial-Temporal Evolution of Ozone Pollution and Its Relationship with El Niño-Southern Oscillation in China from 2015 to 2020

Funds: Natural Science Foundation of Shandong Province, China (No.ZR2020MD016)
  • 摘要: 为研究2015—2020年我国近地面臭氧(O3)污染时空演化特征以及厄尔尼诺-南方涛动(ENSO)对我国O3污染的影响,本文基于2015—2020年我国近1 500个监测站点的O3浓度数据(不包括港澳台地区数据),综合运用空间自相关、热点分析、异常值分析及回归分析,研究2015—2020年我国O3污染的时空演化、浓度异常特征及其与ENSO事件和气象因素的关系. 结果表明:①2015—2019年我国O3污染集聚效应不断增强,但2020年显著降低. ②我国O3浓度呈先升高(2015—2018年)后下降(2018—2020年)的特征,2017年、2018年O3年均浓度分别较上一年升高8.72%、1.76%,2019年、2020年O3年均浓度分别较上一年下降3.60%、3.66%. 除2019年、2020年外,O3浓度高值聚集区站点的O3浓度峰值和高值天数(日均值大于120 μg/m3的天数)均大于O3浓度低值聚集区站点. ③O3高浓度时期为每年的4—10月. O3高浓度区域春、夏两季以华北为核心,秋季向华南和东南地区转移. ④回归分析表明,我国O3浓度正异常与ENSO负相拉尼娜相关,O3浓度负异常与ENSO正相厄尔尼诺相关. 我国东南部O3浓度异常主要受ENSO期间太阳辐射异常和降水异常的影响,而西部和北部地区O3浓度异常主要受ENSO期间风速异常的影响. 研究显示,2015—2020年我国O3平均浓度呈先升高后降低的变化趋势,O3高浓度时期以春、夏两季为主,O3高浓度区域随季节而发生变化,且不同区域O3污染变化特征不同,ENSO对我国不同区域O3污染的影响机制不同.

     

  • 图  1  我国空气质量地面监测站点

    审图号:GS京(2023)0895号. 下同.

    Figure  1.  Air quality monitoring sites in China

    图  2  2015—2020年我国O3浓度冷点、热点分布情况

    Figure  2.  Hot and cold spots of O3 annual concentrations in China from 2015 to 2020

    图  3  2015—2020年冷热点代表站点O3浓度时间序列

    Figure  3.  Time series of daily average concentration of O3 at representative cold and hot spots from 2015 to 2020

    图  4  2015—2020年3月、6月、9月、12月我国9个区域内所有站点O3月均浓度的箱线图

    Figure  4.  Box and whisker plots for monthly mean O3 concentrations at all stations within the nine regions of China in March, June, September and December from 2015 to 2020

    表  1  2015—2020年中国O3浓度全局Moran′s I值

    Table  1.   Global Moran′s I of O3 concentrations in China from 2015 to 2020

    年份 全局Moran′s I Z(I)
    2015 0.39 23.86
    2016 0.40 25.25
    2017 0.53 33.58
    2018 0.55 35.16
    2019 0.59 38.68
    2020 0.49 31.37
    下载: 导出CSV

    表  2  2015—2020年我国O3-8 h浓度峰值、谷值及高值情况

    Table  2.   Peak, valley and high values of O3-8 h pollution from 2015 to 2020 in China

    年份峰值谷值峰值时间高值(>120 μg/m3)
    O3-8 h浓度/
    (μg/m3)
    日期O3-8 h浓度/
    (μg/m3)
    日期首峰时间末峰时间春季夏季秋季冬季
    天数频率天数频率天数频率天数频率
    2015155.502015年5月27日34.272015年12月22日2015年5月27日2015年9月20日160.17120.1350.0500
    2016155.662016年6月9日39.342016年12月25日2016年5月11日2016年11月15日160.17230.2590.1000
    2017181.382017年5月28日38.492017年12月14日2017年5月28日2017年9月18日500.54330.360000
    2018159.182018年4月18日35.052018年12月10日2018年4月18日2018年10月4日430.47470.456000
    2019162.302019年9月28日37.572019年1月10日2019年5月23日2019年9月28日360.39380.4140.0400
    2020156.702020年4月29日37.542020年1月2日2020年4月29日2020年9月6日220.24120.1340.0400
    下载: 导出CSV

    表  3  Niño3.4指数与O3月均浓度异常的回归分析

    Table  3.   Regression analysis of Niño3.4 index and abnormal O3 monthly mean concentrations

    区域Lag-0Lag-1Lag-2
    负值占比/%正值占比/%负值占比/%正值占比/%负值占比/%正值占比/%
    西北地区71.3320.2870.6320.9869.2322.38
    内蒙古自治区69.5719.5771.7417.3976.0913.04
    东北地区46.1149.1053.2941.9256.2938.92
    青藏地区48.2837.0337.9348.2841.3844.83
    华中地区62.1229.1766.2925.0073.1118.18
    华北地区65.9719.7574.3711.3475.6310.08
    西南地区60.3323.9156.5227.7257.0727.17
    华南地区85.6311.8891.256.2595.002.50
    华东地区51.8833.0854.8930.0860.5324.44
    注:Lag-0、Lag-1和Lag-2分别代表O3浓度月均异常值不滞后、滞后Niño3.4指数一个月、滞后Niño3.4指数两个月.
    下载: 导出CSV
  • [1] WANG T,XUE L K,BRIMBLECOMBE P,et al.Ozone pollution in China:a review of concentrations,meteorological influences,chemical precursors,and effects[J].Science of the Total Environment,2017,575:1582-1596. doi: 10.1016/j.scitotenv.2016.10.081
    [2] 李慧,王淑兰,张文杰,等.京津冀及周边地区“2+26”城市空气质量特征及其影响因素[J].环境科学研究,2021,34(1):172-184.

    LI H,WANG S L,ZHANG W J,et al.Characteristics and influencing factors of urban air quality in Beijing-Tianjin-Hebei and its surrounding areas (‘2+26’ cities)[J].Research of Environmental Sciences,2021,34(1):172-184.
    [3] LIU X J,XU W,DUAN L,et al.Atmospheric nitrogen emission,deposition,and air quality impacts in China:an overview[J].Current Pollution Reports,2017,3(2):65-77. doi: 10.1007/s40726-017-0053-9
    [4] 姜华,常宏咪.我国臭氧污染形势分析及成因初探[J].环境科学研究,2021,34(7):1576-1582.

    JIANG H,CHANG H M.Analysis of China's ozone pollution situation,preliminary investigation of causes and prevention and control recommendations[J].Research of Environmental Sciences,2021,34(7):1576-1582.
    [5] 栗泽苑,杨雷峰,华道柱,等.2013—2018年中国近地面臭氧浓度空间分布特征及其与气象因子的关系[J].环境科学研究,2021,34(9):2094-2104.

    LI Z Y,YANG L F,HUA D Z,et al.Spatial pattern of surface ozone and its relationship with meteorological variables in China during 2013-2018[J].Research of Environmental Sciences,2021,34(9):2094-2104.
    [6] 张涵,姜华,高健,等.PM2.5与臭氧污染形成机制及协同防控思路[J].环境科学研究,2022,35(3):611-620.

    ZHANG H,JIANG H,GAO J,et al.Formation mechanism and management strategy of cooperative control of PM2.5 and O3[J].Research of Environmental Sciences,2022,35(3):611-620.
    [7] ZHAO S P,YIN D Y,YU Y,et al.PM2.5 and O3 pollution during 2015-2019 over 367 Chinese cities:spatiotemporal variations,meteorological and topographical impacts[J].Environmental Pollution,2020,264:114694. doi: 10.1016/j.envpol.2020.114694
    [8] WEI J,LI Z Q,LI K,et al.Full-coverage mapping and spatiotemporal variations of ground-level ozone (O3) pollution from 2013 to 2020 across China[J].Remote Sensing of Environment,2022,270:112775. doi: 10.1016/j.rse.2021.112775
    [9] 曾贤刚,阮芳芳,姜艺婧.中国臭氧污染的空间分布和健康效应[J].中国环境科学,2019,39(9):4025-4032. doi: 10.3969/j.issn.1000-6923.2019.09.051

    ZENG X G,RUAN F F,JIANG Y J.Spatial distribution and health effects of ozone pollution in China[J].China Environmental Science,2019,39(9):4025-4032. doi: 10.3969/j.issn.1000-6923.2019.09.051
    [10] WANG Y H,GAO W K,WANG S,et al.Contrasting trends of PM2.5 and surface-ozone concentrations in China from 2013 to 2017[J].National Science Review,2020,7(8):1331-1339. doi: 10.1093/nsr/nwaa032
    [11] LI K,JACOB D J,LIAO H,et al.Anthropogenic drivers of 2013-2017 trends in summer surface ozone in China[J].PNAS,2019,116(2):422-427. doi: 10.1073/pnas.1812168116
    [12] KALSOOM U,WANG T J,MA C Q,et al.Quadrennial variability and trends of surface ozone across China during 2015-2018:a regional approach[J].Atmospheric Environment,2021,245:117989. doi: 10.1016/j.atmosenv.2020.117989
    [13] DANG R J,LIAO H,FU Y.Quantifying the anthropogenic and meteorological influences on summertime surface ozone in China over 2012-2017[J].Science of the Total Environment,2021,754:142394. doi: 10.1016/j.scitotenv.2020.142394
    [14] DING D,XING J,WANG S X,et al.Impacts of emissions and meteorological changes on China's ozone pollution in the warm seasons of 2013 and 2017[J].Frontiers of Environmental Science & Engineering,2019,13(5):1-9.
    [15] LI G H,BEI N F,CAO J J,et al.Widespread and persistent ozone pollution in eastern China during the non-winter season of 2015:observations and source attributions[J].Atmospheric Chemistry and Physics,2017,17(4):2759-2774. doi: 10.5194/acp-17-2759-2017
    [16] LIU Y M,WANG T.Worsening urban ozone pollution in China from 2013 to 2017.part 1:the complex and varying roles of meteorology[J].Atmospheric Chemistry and Physics,2020,20(11):6305-6321. doi: 10.5194/acp-20-6305-2020
    [17] LIU Y M,WANG T.Worsening urban ozone pollution in China from 2013 to 2017.part 2:the effects of emission changes and implications for multi-pollutant control[J].Atmospheric Chemistry and Physics,2020,20(11):6323-6337. doi: 10.5194/acp-20-6323-2020
    [18] ZHAO Z J,WANG Y X.Influence of the West Pacific subtropical high on surface ozone daily variability in summertime over eastern China[J].Atmospheric Environment,2017,170:197-204. doi: 10.1016/j.atmosenv.2017.09.024
    [19] LI K,JACOB D J,SHEN L,et al.Increases in surface ozone pollution in China from 2013 to 2019:anthropogenic and meteorological influences[J].Atmospheric Chemistry and Physics,2020,20(19):11423-11433. doi: 10.5194/acp-20-11423-2020
    [20] CHEN Z Y,LI R Y,CHEN D L,et al.Understanding the causal influence of major meteorological factors on ground ozone concentrations across China[J].Journal of Cleaner Production,2020,242:118498. doi: 10.1016/j.jclepro.2019.118498
    [21] YANG Z,YANG J,LI M M,et al.Nonlinear and lagged meteorological effects on daily levels of ambient PM2.5 and O3:evidence from 284 Chinese cities[J].Journal of Cleaner Production,2021,278:123931. doi: 10.1016/j.jclepro.2020.123931
    [22] WIE J,MOON B K,YEH S W,et al.La Niña-related tropospheric column ozone enhancement over East Asia[J].Atmospheric Environment,2021,261:118575. doi: 10.1016/j.atmosenv.2021.118575
    [23] YANG Y,LI M Y,WANG H L,et al.ENSO modulation of summertime tropospheric ozone over China[J].Environmental Research Letters,2022,17(3):034020. doi: 10.1088/1748-9326/ac54cd
    [24] WANG X H,ZHONG S Y,BIAN X D,et al.Impact of 2015-2016 El Niño and 2017-2018 La Niña on PM2.5 concentrations across China[J].Atmospheric Environment,2019,208:61-73. doi: 10.1016/j.atmosenv.2019.03.035
    [25] XU L,YU J Y,SCHNELL J L,et al.The seasonality and geographic dependence of ENSO impacts on US surface ozone variability[J].Geophysical Research Letters,2017,44(7):3420-3428. doi: 10.1002/2017GL073044
    [26] DONG L,CHEN B,HUANG Y,et al.Analysis on the characteristics of air pollution in China during the COVID-19 outbreak[J].Atmosphere,2021,12(2):205. doi: 10.3390/atmos12020205
    [27] ZHANG X H,TANG M L,GUO F J,et al.Associations between air pollution and COVID-19 epidemic during quarantine period in China[J].Environmental Pollution,2021,268:115897. doi: 10.1016/j.envpol.2020.115897
    [28] ETHAN C J,MOKOENA K K,YU Y.Air pollution status in 10 mega-cities in China during the initial phase of the COVID-19 outbreak[J].International Journal of Environmental Research and Public Health,2021,18(6):3172. doi: 10.3390/ijerph18063172
    [29] ZHAO S P,YU Y,YIN D Y,et al.Annual and diurnal variations of gaseous and particulate pollutants in 31 provincial capital cities based on in situ air quality monitoring data from China National Environmental Monitoring Center[J].Environment International,2016,86:92-106. doi: 10.1016/j.envint.2015.11.003
    [30] HERSBACH H,BELL B,BERRISFORD P,et al.The ERA5 global reanalysis[J].Quarterly Journal of the Royal Meteorological Society,2020,146(730):1999-2049. doi: 10.1002/qj.3803
    [31] SAHA S,MOORTHI S,WU X R,et al.The NCEP climate forecast system version 2[J].Journal of Climate,2014,27(6):2185-2208. doi: 10.1175/JCLI-D-12-00823.1
    [32] SHI G Q,LIU J X,ZHONG X N.Spatial and temporal variations of PM2.5 concentrations in Chinese cities during 2015-2019[J].International Journal of Environmental Health Research,2021,32(12):1-13.
    [33] ANSELIN L.Local indicators of spatial association-LISA[J].Geographical Analysis,2010,27(2):93-115. doi: 10.1111/j.1538-4632.1995.tb00338.x
    [34] GOODCHILD M,HAINING R,WISE S.Integrating GIS and spatial data analysis:problems and possibilities[J].International Journal of Geographical Information Systems,1992,6(5):407-423. doi: 10.1080/02693799208901923
    [35] 周明卫,康平,汪可可,等.2016—2018年中国城市臭氧浓度时空聚集变化规律[J].中国环境科学,2020,40(5):1963-1974. doi: 10.3969/j.issn.1000-6923.2020.05.013

    ZHOU M W,KANG P,WANG K K,et al.The spatio-temporal aggregation pattern of ozone concentration in China from 2016 to 2018[J].China Environmental Science,2020,40(5):1963-1974. doi: 10.3969/j.issn.1000-6923.2020.05.013
    [36] HE G J,PAN Y H,TANAKA T.The short-term impacts of COVID-19 lockdown on urban air pollution in China[J].Nature Sustainability,2020,3(12):1005-1011. doi: 10.1038/s41893-020-0581-y
    [37] CHEN Y,ZHANG S M,PENG C,et al.Impact of the COVID-19 pandemic and control measures on air quality and aerosol light absorption in southwestern China[J].Science of the Total Environment,2020,749:141419. doi: 10.1016/j.scitotenv.2020.141419
    [38] 郭欣瞳,宋宏权,梁留科,等.2015—2017年中国臭氧浓度时空变化特征[J].气象与环境科学,2020,43(3):41-50.

    GUO X T,SONG H Q,LIANG L K,et al.Spatial and temporal variations of ozone concentration in China during 2015-2017[J].Meteorological and Environmental Sciences,2020,43(3):41-50.
    [39] 黄小刚,赵景波,曹军骥,等.中国城市O3浓度时空变化特征及驱动因素[J].环境科学,2019,40(3):1120-1131.

    HUANG X G,ZHAO J B,CAO J J,et al.Spatial-temporal variation of ozone concentration and its driving factors in China[J].Environmental Science,2019,40(3):1120-1131.
    [40] REN J,HAO Y F,SIMAYI M,et al.Spatiotemporal variation of surface ozone and its causes in Beijing,China since 2014[J].Atmospheric Environment,2021,260:118556. doi: 10.1016/j.atmosenv.2021.118556
    [41] YANG G F,LIU Y H,LI X N.Spatiotemporal distribution of ground-level ozone in China at a city level[J].Scientific Reports,2020,10:7229. doi: 10.1038/s41598-020-64111-3
    [42] YIM S H L,HOU X,GUO J,et al.Contribution of local emissions and transboundary air pollution to air quality in Hong Kong during El Niño-Southern Oscillation and heatwaves[J].Atmospheric Research,2019,218:50-58. doi: 10.1016/j.atmosres.2018.10.021
    [43] YIN Z C,CAO B F,WANG H J.Dominant patterns of summer ozone pollution in eastern China and associated atmospheric circulations[J].Atmospheric Chemistry and Physics,2019,19(22):13933-13943. doi: 10.5194/acp-19-13933-2019
    [44] ZENG L,YANG Y,WANG H,et al.Intensified modulation of winter aerosol pollution in China by El Niño with short duration[J].Atmospheric Chemistry and Physics,2021,21(13):10745-10761. doi: 10.5194/acp-21-10745-2021
    [45] SUN J R,LI H Y,ZHANG W J,et al.Modulation of the ENSO on winter aerosol pollution in the eastern region of China[J].Journal of Geophysical Research:Atmospheres,2018,123(21):11952-11969. doi: 10.1029/2018JD028534
    [46] LI M Y,YANG Y,WANG P Y,et al.Impacts of strong El Niño on summertime near-surface ozone over China[J].Atmospheric and Oceanic Science Letters,2022,15(4):100193. doi: 10.1016/j.aosl.2022.100193
    [47] 赵恺辉,包云轩,黄建平,等.华南地区春季平流层入侵对对流层低层臭氧影响的模拟研究[J].大气科学,2019,43(1):75-86.

    ZHAO K H,BAO Y X,HUANG J P,et al.A modeling study of the impact of stratospheric intrusion on ozone enhancement in the lower troposphere in South China[J].Chinese Journal of Atmospheric Sciences,2019,43(1):75-86.
  • 加载中
图(4) / 表(3)
计量
  • 文章访问数:  221
  • HTML全文浏览量:  100
  • PDF下载量:  121
  • 被引次数: 0
出版历程
  • 收稿日期:  2022-06-21
  • 修回日期:  2022-10-31

目录

    /

    返回文章
    返回